For its many useful properties, including second and third-order optical nonlinearity as well as electro-optic control, lithium niobate is considered an important potential microcomb material. Here, a soliton microcomb is demonstrated in a monolithic high-Q lithium niobate resonator. Besides the demonstration of soltion mode locking, the photorefractive effect enables mode locking to self-start and soliton switching to occur bi-directionally. Second-harmonic generation of the soliton spectrum is also observed, an essential step for comb self-referencing. The Raman shock time constant of lithium niobate is also determined by measurement of soliton self-frequency-shift. Besides the considerable technical simplification provided by a self-starting soliton system, these demonstrations, together with the electro-optic and piezoelectric properties of lithium niobate, open the door to a multi-functional microcomb providing f-2f generation and fast electrical control of optical frequency and repetition rate, all of which are critical in applications including time keeping, frequency synthesis/division, spectroscopy and signal generation.
arXiv:1812.09610v1 [physics.optics]Abstract In this supplement detailed information is provided on the following: the device design, the experimental setup, the numeric modeling of soliton comb generation with analysis of self-starting mode locking, and the characterization of key device parameters. * These two authors contributed equally. † Electronic