Non-vacuum electrodeposition (ED) was used to prepare a biaxially textured Gd 2 Zr 2 O 7 (GZO) and GZO/Gd 2 O 3 (GO) buffer layer on a Ni-W substrate. The YBa 2 Cu 3 O 7-d (YBCO) superconductor was deposited by pulsed-laser deposition (PLD) on a simplified ED-GZO and ED-GZO/ED-GO buffer layer. The buffer layers and YBCO superconductor were characterized by X-ray diffraction (including h/2h, pole figure, omega scans, and phi scans) and atomic force microscopy. Full-width at half maximum values of the omega (x) and phi (U) scans of the electrodeposited GZO and GZO/GO layer were better than those of the Ni-W base substrate. At 77 K and a self-magnetic field, the critical current density of PLD YBCO on the electrodeposited-based buffer layer was 3.3 · 10 6 A/cm 2 , using the field criterion of 1 lV/cm.