“…2D materials have shown to exhibit extremely high nonlinear optical susceptibilities, with several nonlinear optical effects observed, including second [5][6][7][8][9][10] and third 9,11,12 harmonic generation (SHG/THG), sum-frequency generation 13 , four-wave mixing [13][14][15] , and high-harmonic generation [16][17][18] . This makes frequency conversion in 2D materials extremely promising, with potential applications to ultrafast pulse characterization 19 , alloptical wavelength conversion for telecommunications 4 , optical imaging 7,13 , quantum information processing 20,21 , nanoscale lightsources 22,23 , among others. In addition, SHG and THG have proven to be a key technique for crystal orientation and characterization of fundamental material properties 12,24 .…”