Graphene-based three-dimensional (3D) magnetic assemblies have attracted great research attention owing to their multiple natures inherited from 3D graphene assemblies and magnetic materials. However, at present, the practical applications of graphene-based magnetic materials are limited by the relative complex synthesis procedure and harsh operation conditions. Hence, a facile and green synthesis strategy is highly desired. Herein, a magnetic graphene aerogel with magnetite nanoparticles in-situ synthesized on the surface of its frameworks was fabricated through a green and facile strategy. The synthesis process was performed in a gentle condition with low energy consumption. The obtained graphene aerogels exhibited superior magnetism with a saturation magnetization of 55.7 emu·g−1. With the merits of well-developed pore structures, high surface area, and robust magnetic property, the obtained composite aerogels exhibited intriguing adsorption and photo-Fenton catalytic degradation performances for the organic dyes in water. Moreover, the utilized graphene aerogels could be recycled from the water due to their effective magnetic separation performance, indicating a promising capability for practical applications in the area of water remediation. We anticipate this synthesis strategy could provide some guidance for the design and development of 3D magnetic assemblies.

A kind of functional composite was prepared by loading silver nanoparticles firmly on the surface of spherical activated carbon, which showed chemical adsorption properties for chemical warfare agents and satisfactory antibacterial activity.