Solution-processed hybrid perovskite of CH3NH3PbI3 (MAPbI3) exhibits an abnormal luminescence behavior at around the tetragonal-orthorhombic phase transition temperature. The combination of time resolved photoluminescence (PL), variable excitation power PL, and variable-temperature X-ray diffraction (XRD) allows us to clearly interpret the abnormal luminescence features in the phase transition region of MAPbI3. Both PL and XRD results unambiguously prove the coexistence of the tetragonal and orthorhombic phases of MAPbI3 in the temperature range of 150 to 130 K. The two luminescence features observed in the orthorhombic phase at T < 130 K originate from free excitons and donor-acceptor-pair (DAP) transitions, respectively. The comprehensive understanding of optical properties upon phase transition in MAPbI3 will benefit the development of new optoelectronic devices.
We study nonlinear Cerenkov radiation generated from a nonlinear photonic crystal waveguide where the nonlinear susceptibility tensor is modulated by the ferroelectric domain. Nonlinear polarization driven by an incident light field may emit coherently harmonic waves at new frequencies along the direction of Cerenkov angles. Multiple radiation spots with different azimuth angles are simultaneously exhibited from such a hexagonally poled waveguide. A scattering involved nonlinear Cerenkov arc is also observed for the first time. Cerenkov radiation associated with quasi-phase matching leads to these novel nonlinear phenomena.
Single solitons are a special limit of more general waveforms commonly referred to as cnoidal waves or Turing rolls. We theoretically and computationally investigate the stability and accessibility of cnoidal waves in microresonators. We show that they are robust and, in contrast to single solitons, can be easily and deterministically accessed in most cases. Their bandwidth can be comparable to single solitons, in which limit they are effectively a periodic train of solitons and correspond to a frequency comb with increased power. We comprehensively explore the three-dimensional parameter space that consists of detuning, pump amplitude, and mode circumference in order to determine where stable solutions exist. To carry out this task, we use a unique set of computational tools based on dynamical system theory that allow us to rapidly and accurately determine the stable region for each cnoidal wave periodicity and to find the instability mechanisms and their time scales. Finally, we focus on the soliton limit, and we show that the stable region for single solitons almost completely overlaps the stable region for both continuous waves and several higher-periodicity cnoidal waves that are effectively multiple soliton trains. This result explains in part why it is difficult to access single solitons deterministically.
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