Impressive properties arise from the atomically thin nature of transition metal dichalcogenide two-dimensional materials. However, being atomically thin limits their optical absorption or emission. Hence, enhancing their photoluminescence by plasmonic nanostructures is critical for integrating these materials in optoelectronic and photonic devices. Typical photoluminescence enhancement from transition metal dichalcogenides is 100-fold, with recent enhancement of 1,000-fold achieved by simultaneously enhancing absorption, emission and directionality of the system. By suspending WSe2 flakes onto sub-20-nm-wide trenches in gold substrate, we report a giant photoluminescence enhancement of ∼20,000-fold. It is attributed to an enhanced absorption of the pump laser due to the lateral gap plasmons confined in the trenches and the enhanced Purcell factor by the plasmonic nanostructure. This work demonstrates the feasibility of giant photoluminescence enhancement in WSe2 with judiciously designed plasmonic nanostructures and paves a way towards the implementation of plasmon-enhanced transition metal dichalcogenide photodetectors, sensors and emitters.
Recent developments in color filtering and display technologies have focused predominantly on high resolution, color vibrancy, high efficiency, and slim dimensions. To achieve these goals, metallic nanostructures have attracted extensive research interest due to their abilities to manipulate the properties of light through surface plasmon resonances. In this paper, we review recent representative developments in plasmonic color engineering at the nanoscale using subwavelength nanostructures, demonstrating their great potential in high-resolution and high-fidelity color rendering, spectral filtering applications, holography, three-dimensional stereoscopic imaging, etc.
Metamaterials open up various exotic means to control electromagnetic waves and among them polarization manipulations with metamaterials have attracted intense attention. As of today, static responses of resonators in metamaterials lead to a narrow-band and single-function operation. Extension of the working frequency relies on multilayer metamaterials or different unit cells, which hinder the development of ultra-compact optical systems. In this work, we demonstrate a switchable ultrathin terahertz quarter-wave plate by hybridizing a phase change material, vanadium dioxide (VO2), with a metasurface. Before the phase transition, VO2 behaves as a semiconductor and the metasurface operates as a quarter-wave plate at 0.468 THz. After the transition to metal phase, the quarter-wave plate operates at 0.502 THz. At the corresponding operating frequencies, the metasurface converts a linearly polarized light into a circularly polarized light. This work reveals the feasibility to realize tunable/active and extremely low-profile polarization manipulation devices in the terahertz regime through the incorporation of such phase-change metasurfaces, enabling novel applications of ultrathin terahertz meta-devices.
We demonstrate a simple, direct measurement of propagation losses in single silver nanowires. Using a waveguiding nanoscale fiber taper for highly efficient launching, propagation surface plasmon polaritons are excited in the silver nanowire with high efficiency. The output intensity as light radiation at the end of the nanowire is quantified with high accuracy and repeatability. A typical propagation loss of 0.41 dB radicalmum (for 633 nm light) in a 260 nm diameter silver nanowire is obtained, which suggests that the propagation loss of a single silver nanowire could be lower than previously reported experimental results and should be much lower than those obtained by theoretical calculations.
Combining the advantages of ultrahigh photon emission rates achievable in the gap surface plasmon polaritons with high extraction decay rates into low-loss nanofibers, we demonstrate theoretically the efficient photon emission of a single dipole emitter and one-dimensional nanoscale guiding in metallic nanorod-coupled nanofilm structures coupled to dielectric nanofibers. We find that total decay rates and surface plasmon polariton channel decay rates orders of magnitude larger than those characteristic of metallic nanofilms alone can be achieved in ultrastrong hot spots of gap plasmons. For the requirement of practical applications, propagating single photons with decay rates of 290γ_{0}-770γ_{0} are guided into the phase-matched low-loss nanofibers. The proposed mechanism promises to have an important impact on metal-based optical cavities, on-chip bright single photon sources and plasmon-based nanolasers.
Palladium diselenide (PdSe2) is an emerging 2D layered material with anisotropic optical/electrical properties, extra‐high carrier mobility, excellent air stability, etc. So far, ultrathin PdSe2 is mainly achieved via mechanical exfoliation from its bulk counterpart, and the direct synthesis is still challenging. Herein, the synthesis of ultrathin 2D PdSe2 on conductive Au foil substrates via a facile chemical vapor deposition route is reported. Intriguingly, an anisotropic growth behavior is detected from the evolution of ribboned flakes with large length/width ratios, which is well explained from the orthorhombic symmetry of PdSe2. A unique even‐layered growth mode from 2 to 20 layers is also confirmed by the perfect combination of onsite scanning tunneling microscopy characterizations, through deliberately scratching the flake edge to expose both even and odd layers. This even‐layered, ribboned 2D material is expected to serve as a perfect platform for exploring unique physical properties, and for developing high‐performance electronic and optoelectronic devices.
Premature ovarian failure (POF) is a refractory disease for clinical treatment with the goal of restoring fertility. In this study, umbilical cord mesenchymal stem cells on a collagen scaffold (collagen/UC-MSCs) can activate primordial follicles in vitro via phosphorylation of FOXO3a and FOXO1. Transplantation of collagen/UC-MSCs to the ovaries of POF patients rescued overall ovarian function, evidenced by elevated estradiol concentrations, improved follicular development, and increased number of antral follicles. Successful clinical pregnancy was achieved in women with POF after transplantation of collagen/UC-MSCs or UC-MSCs. In summary, collagen/UC-MSC transplantation may provide an effective treatment for POF.
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