A 3D printer based slot‐die coater is developed as a lab‐to‐fab translation tool for solution‐processed solar cells. The modified 3D printer is used to develop the printing process for potential use in large scale roll‐to‐roll production. Fabrication of a 47.3 cm2 organic solar cell module with 4.56% efficiency and printed perovskite solar cells with 11.6% efficiency are demonstrated.

No abstract

Recently, many kinds of printing processes have been studied to fabricate perovskite solar cells (PeSCs) for mass production. Among them, slot-die coating is a promising candidate for roll-to-roll processing because of high-throughput, easy module patterning, and a premetered coating system. In this work, we employed mixed lead precursors consisting of PbAc and PbCl to fabricate PeSCs via slot-die coating. We observed that slot-die-coated perovskite films based on the mixed lead precursors exhibited well-grown and uniform morphology, which was hard to achieve by using only a single lead source. Consequently, PeSCs made with this precursor system showed improved device performance and reproducibility over single PbAc. Lastly, a large-area module with an active area of 10 cm was fabricated with a power conversion efficiency of 8.3%.