In this work, a sensitive deep ultraviolet (DUV) light photodetector based on inorganic and lead-free Cs 3 Cu 2 I 5 crystalline film derived by a solution method was reported. Optoelectronic characterization revealed that the perovskite device exhibited nearly no sensitivity to visible illumination with wavelength of 405 nm but exhibited pronounced sensitivity to both DUV and UV light illumination with response speeds of 26.2/49.9 ms for rise/fall time. The I light /I dark ratio could reach 127. What is more, the responsivity and specific detectivity were calculated to be 64.9 mA W −1 and 6.9 × 10 11 Jones, respectively. In addition, the device could keep its photoresponsivity after storage in air environment for a month. It is also found that the capability of Cs 3 Cu 2 I 5 crystalline film device can readily record still DUV image with acceptable resolution. The above results confirm that the DUV photodetector may hold great potential for future DUV optoelectronic device and systems.
In this study, a sensitive infrared photodetector (IRPD) composed of a germanium nanocones (GeNCs) array and PdSe2 multilayer is presented, which is obtained by a straightforward selenization approach. The as‐assembled PdSe2/GeNCs hybrid heterojunction exhibits obvious photovoltaic behavior to 1550 nm illumination, which renders the IRPD a self‐driven device without external power supply. Further device analysis reveals that the PdSe2/GeNCs hybrid based IRPD exhibits high sensitivity to 1350, 1550, and 1650 nm illumination with excellent stability and reproducibility. The responsivity and external quantum efficiency is as high as 530.2 mA W−1 and 42.4%, respectively. Such a relatively good device performance is related to the strong light trapping effect of GeNCs array, according to the theoretical simulation based on finite‐difference time‐domain. It is also found that the IRPD shows an abnormal sensitivity to IR illumination with a wavelength of 2200 nm. Finally, the present individual IRPD can also record the simple “F” image produced by 1550 nm, suggesting the promising application of the PdSe2/GeNCs hybrid device in future infrared optoelectronic systems.
In this study, a highly sensitive and self‐driven near‐infrared (NIR) light photodetector based on PdSe2/pyramid Si heterojunction arrays, which are fabricated through simple selenization of predeposited Pd nanofilm on black Si, is demonstrated. The as‐fabricated hybrid device exhibits excellent photoresponse performance in terms of a large on/off ratio of 1.6 × 105, a responsivity of 456 mA W−1, and a high specific detectivity of up to 9.97 × 1013 Jones under 980 nm illumination at zero bias. Such a relatively high sensitivity can be ascribed to the light trapping effect of the pyramid microstructure, which is confirmed by numerical modeling based on finite‐difference time domain. On the other hand, thanks to the broad optical absorption properties of PdSe2, the as‐fabricated device also exhibits obvious sensitivity to other NIR illuminations with wavelengths of 1300, 1550, and 1650 nm, which is beyond the photoresponse range of Si‐based devices. It is also found that the PdSe2/pyramid Si heterojunction device can also function as an NIR light sensor, which can readily record both “tree” and “house” images produced by 980 and 1300 nm illumination, respectively.
In this study, we have developed a high-sensitivity, near-infrared photodetector based on PdSe2/GaAs heterojunction, which was made by transferring a multilayered PdSe2 film onto a planar GaAs. The as-fabricated PdSe2/GaAs heterojunction device exhibited obvious photovoltaic behavior to 808 nm illumination, indicating that the near-infrared photodetector can be used as a self-driven device without external power supply. Further device analysis showed that the hybrid heterojunction exhibited a high on/off ratio of 1.16×105 measured at 808 nm under zero bias voltage. The responsivity and specific detectivity of photodetector were estimated to be 171.34 mA/W and 2.36×1011 Jones, respectively. Moreover, the device showed excellent stability and reliable repeatability. After 2 months, the photoelectric characteristics of the near-infrared photodetector hardly degrade in air, attributable to the good stability of the PdSe2. Finally, the PdSe2/GaAs-based heterojunction device can also function as a near-infrared light sensor.
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