Although water quality has been improved in the last
two decades,
water pollution by organic contaminants has remained a non-negligible
issue in China. It is worthwhile to assess human exposure risks to
waterborne organic contaminants and find the relation between them
and carcinogenic risks. This work reviews the spatiotemporal patterns
of water quality and typical organic contaminants in drinking water
sources (i.e., surface water, groundwater, and tap water) in relation
to age-standardized incidences of total cancers in China over 16 years.
The improvement of water quality for drinking water sources seemed
to produce a positive effect in reducing incidences of polluted water-related
diseases and digestive system cancers. Although the total accumulative
lifetime cancer risk for residents through water drinking and dermal
exposure to typical carcinogenic organic contaminants was lower than
the latest incidences of digestive system cancers and total cancers
excluding lung cancer published by the Chinese government, their similar
spatial patterns indicated that this exposure should be considered
as one of potential factors for carcinogenic risks. Finally, further
efforts to explore the correlation between human exposure to organic
contaminants in water and related health effects on a long-term basis
should be helpful for establishing and implementing feasible management
strategies to reduce disease burdens.
Activated carbon (AC) amendment is an effective strategy for remediating contaminated sediment by hydrophobic organic chemicals. Reductions of porewater chemical concentrations have been used for estimating recommended AC dose for effective sediment remediation, but the AC dose may have large uncertainties resulting from site-specific parameters. The present study examined sediment−water diffusion flux as an alternative assessment parameter by correlating diffusion fluxes of organophosphorus flame retardants (OPFRs) and polybrominated diphenyl ethers (PBDEs) with AC doses. AC at doses of 8−36% substantially reduced sediment porewater concentrations and diffusion fluxes of the target chemicals. Diffusion fluxes of OPFRs and PBDEs normalized by their corresponding sediment concentrations significantly correlated with total organic carbon contents (r 2 = 0.57−0.93). A model was established to estimate the required AC dose for effective sediment amendment from the diffusion flux and sediment concentration of a target chemical. Using contaminated sediment in a typical e-waste recycling zone, the AC doses (0.1 ± 1.3−12.8 ± 0.3%) required to reduce 90% of diffusion fluxes for tri-n-butyl phosphate and BDE-17 were within the recommended range (1.9 ± 3.6−5.6 ± 8.3%) in lowering porewater concentrations by the same magnitude. This finding suggested the feasibility of the new model in supporting sediment remediation.
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