This paper reports the results obtained for the degradation of acetaldehyde by an atmospheric plasma corona discharge working in a pulsed regime. It was shown that a few hundred ppm of acetaldehyde diluted in a pure N 2 gas flow can be removed up to 80% by a discharge fed with an electric power lower than 1 W. Under the same conditions, adding up to 5% of O 2 allowed the removal of up to 95% of the initial acetaldehyde. The main identified end products were CO 2 , CO and methanol. A quasi-homogeneous zero-dimensional chemical model was developed to investigate the respective efficiency of the discharge and post-discharge periods in the global removal of the pollutant. The identified main pathways of acetaldehyde degradation were quenching of N 2 metastable states during plasma pulses and oxidation by O and OH radicals during the post-discharge. This latter contribution increased with input power because of ozone accumulation in the gas mixture acting as an additional oxygen reservoir.
In Dielectric Barrier Discharges (DBDs), the control of the power transfer, from the low-voltage static converter to the high voltage DBD, is strongly affected by the parasitic capacitive effects of the step-up transformer. Minimizing these capacitances is of major importance and this paper aims to establish and validate analytical expressions in order to predict the values of the parasitic capacitances of high ratio, step-up transformers, according to different windings arrangements using cylindrical conductors. Afterward, experimental validations are performed on three transformers which have been realized according to same specifications, in order to show the accuracy of the method and to understand the influence the winding arrangements on the capacitive parasitic effects.
This paper proposes a design approach of an electrical power supply intended to offer an especially well-suited supply mode, through the efficient control of the current injected into a DBD setup. The proposed topology is aimed at controlling the operating point of the electrical discharge, thereby allowing favoring the homogeneous regime, and maximizing the electrical power injected into the plasma. The power supply structure is designed on the basis of causality criteria and of an analytical analysis of the electrical waveforms, which are derived from an equivalent circuit model of the DBD. Design issues of this electrical generator are detailed and experimental analysis of its operation, together with actual performances are presented. A very good agreement is obtained by comparing simulation and experiments. Effective ability to control the power transfers by means of its two degrees of freedom (current magnitude and frequency) is highlighted.
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