Polycrystalline Sr2Fe1−xAlxMoO6 compounds with x=0, 0.05, 0.10, 0.15, and 0.30 were fabricated and their low-field magnetoresistance (LFMR) performance studied. The LFMR was greatly enhanced as x increased from nil to 0.15, and its origin was found to be intragranular spin-dependent scattering. The replacement of Fe by Al weakened the antiferromagnetic exchange in the antiphase boundary arising from the antisite defect and acted as a barrier for electron transport along the Mo–O–Fe–O–Mo–O–Fe chain in the ferromagnetic segregation and weakened the ferromagnetic exchange. When the external magnetic field was applied, the spin in the antiphase boundary appeared to align more easily to the external field after Al doping and the transport of the electron was easier due to the weakening of the double exchange barrier.

Cobalt-copper nonlocal spin valves are fabricated by shadow evaporation through nanoscale masks. The thickness of Co electrodes is varied and the spin diffusion length of the Cu channel is determined. Short spin diffusion lengths are found in devices with thick ͑Ͼ20 nm͒ Co layers. Co impurities are introduced into the Cu channel in the shadow evaporation process during the fabrication, and the impurities cause spin-flip scattering. The amount of Co impurities can be reduced by decreasing the thicknesses of Co electrodes. Spin diffusion lengths of ϳ400 nm at 295 K and ϳ800 nm at 4.2 K are measured in devices with thin ͑Ͻ10 nm͒ Co layers.