Carbon fiber (CF) nonwoven fabric possesses excellent chemical resistance, remarkable electrical properties, and low density, but its mechanical strength must be enhanced to facilitate its application. Therefore, a flexible compound nonwoven fabric (CEF-NF) consisting of CF and a bicomponent polypropylene/polyethylene core/sheath fiber (known as ESF) was prepared using a 2-step wet papermaking/ thermal bonding process. Scanning electron microscopy observations indicated that the CEF-NF fibrous network could be strengthened without blocking its pores by using a heat-pressing temperature falling between the melting regions of the sheath polyethylene and core polypropylene. Additionally, uniaxial tensile experiments were conducted to investigate the failure mode and tensile properties of the CEF-NF by varying the thermal bonding and structural parameters. The results showed that 3 failure modes of fiber physical contact separation, thermal bond breakage, and ESF fracture emerged and could be defined based on the variation in the heat-pressing temperature. The tensile strength of the CEF-NF was improved with increasing thermal bonding and structural parameters. Under a set of process parameters, ie, 180°C heat-pressing temperature, 6-MPa heat-pressing pressure, 40 wt% ESF mass fraction, and 40-gsm areal density, the tensile strength of CEF-NF reached 5.7 MPa, which is much higher than that of pure CF nonwoven fabric.
In this work, we propose a facile method for manufacturing a three-dimensional copper foil-powder sintering current collector (CFSCC) for a silicon-based anode lithium-ion battery. We found that the CFSCC is suitable as a silicon-based paste electrode, and the paste-like electrodes are commonly used in industrial production. Compared with flat current collectors, the CFSCC better constrained the silicon volume change during the charging-discharging process. The capacitance of electrodes with CFSCC remained as high as 92.2% of its second cycle after 40 cycles, whereas that of electrodes with a flat current collector only remained at 50%.
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