Molecular electronic control over plasmons offers a promising route for on-chip integrated molecular plasmonic devices for information processing and computing. To move beyond the currently available technologies and to miniaturize plasmonic devices, molecular electronic plasmon sources are required. Here, we report on-chip molecular electronic plasmon sources consisting of tunnel junctions based on self-assembled monolayers sandwiched between two metallic electrodes that excite localized plasmons, and surface plasmon polaritons, with tunnelling electrons. The plasmons originate from single, diffraction-limited spots within the junctions, follow power-law distributed photon statistics, and have well-defined polarization orientations. The structure of the self-assembled monolayer and the applied bias influence the observed polarization. We also show molecular electronic control of the plasmon intensity by changing the chemical structure of the molecules and by bias-selective excitation of plasmons using molecular diodes.S urface plasmon polaritons (SPPs) confine and enhance local electromagnetic fields near surfaces of metallic nanostructures at optical frequencies and have the ability to propagate along subdiffractive metallic waveguides, thereby opening up new perspectives for integrated optoelectronic circuits at the nanoscale 1-4 . However, almost all these applications use large external light sources such as monochromatic lasers. To minimize the size of the light sources and ultimately the size of the plasmonic devices, plasmons have been excited on-chip using electrically driven light sources such as (organic) light-emitting diodes (LEDs) 5-8 , laser diodes 9 , silicon spheres 10 and single carbon nanotubes 11 instead of bulky lasers. Surface plasmons have also been directly excited by tunnelling electrons in metal-insulator-metal junctions based on metal oxides 12-14 or scanning tunnelling microscopes (STMs) using vacuum or molecular tunnelling barriers [15][16][17][18][19][20][21][22][23][24][25] . During the tunnelling process, most of the electrons tunnel elastically, but some tunnel inelastically and couple to a plasmon mode. Direct excitation of plasmons by tunnelling electrons is attractive because not only is no background light generated but potentially it is also fast 26 (on the timescale of quantum tunnelling) as no slow electron-hole recombination processes are required as is the case for electroluminescent (nano)light sources 5-11 . Here, we report a direct electronic plasmon source based on molecular tunnel junctions operating via throughmolecular-bond tunnelling, where the plasmonic properties can be electrically controlled at the molecular level (without the need for optical antennas 27,28 ).In molecular electronic devices, the tunnelling barrier height is defined by the electronic energy levels of the molecule(s) bridging two electrodes. The tunnelling barrier width is defined by the length of the bridging molecule. Hence, the tunnelling gaps in molecular electronic devices are always exact...
A highly
efficient nanocavity formed by optically coupled nanostructures
is achieved by optimization of the collective Mie resonances in a
one-dimensional array of semiconductor nanoparticles. Analysis of
quasi-normal multipole modes enables us to reveal the close relation
between the collective Mie resonances and Van Hove singularities.
On the basis of these concepts, we experimentally demonstrate a directional
GaAs nanolaser at cryogenic temperatures with well-defined, in-plane
emission, which, moreover, can be controlled by selective excitation.
The lasing threshold is shown to be significantly reduced by optimizing
the interparticle gap such that the optimal near-field confinement
is achieved at a resonant wavelength corresponding to the highest
gain of GaAs. We show that the lasing performance of this nanolaser
is orders of magnitude better than a nanowire-based laser of the same
dimensions. The present work provides design guidelines for high performance
in-plane emission nanolasers, which may find applications in future
photonic integrated circuits.
In this paper, symmetric and asymmetric tapering on the arms of the gammadion nanostructure is proposed to enhance both local field distribution and extinction difference (ED). The asymmetric tapered gammadion with tapering fraction (TF) of 0.67 is seen to have the largest ED and spatial local field distribution, producing a large wavelength shift of more than 50 percent as compared to the untapered gammadion nanostructures when immersed in a solution of actin molecules and filaments. The optical chirality, ζ shows that the larger local field amplitudes produced by the asymmetric designs increases the rate of chiral molecules excitation. This enhanced field is strongly rotating and highly sensitive to single molecules and larger filaments. Here, we show that the ED, optical chirality, sensitivity and rate of chiral molecules excitation can be improved by incorporating asymmetric designs into chiral gammadion nanostructures through tapering.
There is an urgent need for industrial Internet of things (IoT) solutions to deploy a smart hydrophone sensor grid to monitor pipeline health and to provide an accurate prediction in the event of any leakage. One solution is to develop an IoT water leakage detection system consisting of an interface to capture acoustic signals from aluminum nitride (AlN)-based micro-machined infrasonic hydrophone sensors that are fed as inputs and predict an approximate leak location as a form of output. Micro-electro-mechanical systems (MEMS) are particularly useful for IoT applications with low power consumption and small device footprint. Data analytics including characterization, pre/post processing are applied to determine the leaks. In this work, we have developed the process flow and algorithm to detect pipe leakage occurrence and pinpoint the location accurately. Our approach can be implemented to detect leaks for different pipe lengths, diameters and materials.
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