[1] This paper provides a review of stratosphere-troposphere exchange (STE), with a focus on processes in the extratropics. It also addresses the relevance of STE for tropospheric chemistry, particularly its influence on the oxidative capacity of the troposphere. After summarizing the current state of knowledge, the objectives of the project Influence of Stratosphere-Troposphere Exchange in a Changing Climate on Atmospheric Transport and Oxidation Capacity (STACCATO), recently funded by the European Union, are outlined. Several papers in this Journal of Geophysical ResearchAtmospheres special section present the results of this project, of which this paper gives an overview. STACCATO developed a new concept of STE in the extratropics, explored the capacities of different types of methods and models to diagnose STE, and identified their various strengths and shortcomings. Extensive measurements were made in central Europe, including the first monitoring over an extended period of time of beryllium-10 ( 10 Be), to provide a suitable database for case studies of stratospheric intrusions and for model validation. Photochemical models were used to examine the impact of STE on tropospheric ozone and the oxidizing capacity of the troposphere. Studies of the present interannual variability of STE and projections into the future were made using reanalysis data and climate models.

No abstract

Rossby wave packets (RWPs) are Rossby waves for which the amplitude has a local maximum and decays to smaller values at larger distances. This review focuses on upper-tropospheric transient RWPs along the midlatitude jet stream. Their central characteristic is the propagation in the zonal direction as well as the transfer of wave energy from one individual trough or ridge to its downstream neighbor, a process called “downstream development.” These RWPs sometimes act as long-range precursors to extreme weather and presumably have an influence on the predictability of midlatitude weather systems. The paper reviews research progress in this area with an emphasis on developments during the last 15 years. The current state of knowledge is summarized including a discussion of the RWP life cycle as well as Rossby waveguides. Recent progress in the dynamical understanding of RWPs has been based, in part, on the development of diagnostic methods. These methods include algorithms to identify and track RWPs in an automated manner, which can be used to extract the climatological properties of RWPs. RWP dynamics have traditionally been investigated using the eddy kinetic energy framework; alternative approaches based on potential vorticity and wave activity fluxes are discussed and put into perspective with the more traditional approach. The different diagnostics are compared to each other and the strengths and weaknesses of individual methods are highlighted. A recurrent theme is the role of diabatic processes, which can be a source for forecast errors. Finally, the paper points to important open research questions and suggests avenues for future research.

No abstract

Hemispheric maps of monthly mean total ozone display distinct waves of low zonal wavenumbers during winter months. In addition, there is a strong and statistically significant spatial correlation between the total ozone perturbation and the temperature perturbation in the lower stratosphere. Previous attempts at an explanation of the correlation appear somewhat unsatisfactory. In the current paper the climatological behavior for southern hemisphere October is investigated. Specifying the dynamics from observations in the linearized stationary ozone continuity equation, one can simulate the lowest wavenumbers of the hemispheric total ozone perturbation. Both vertical and horizontal advection substantially contribute to the total ozone perturbation, with significantly different patterns each. A conceptual picture for the correlation is developed, which accounts for both advection contributions. The slopes of lower stratospheric zonal mean potential temperature and ozone mixing ratio turn out to be important. Furthermore, the feasibility of a Matsuno‐type model for the waves in total ozone is shown.

Abstract. During SPURT (Spurenstofftransport in derTropopausenregion, trace gas transport in the tropopause region) we performed measurements of a wide range of trace gases with different lifetimes and sink/source characteristics in the northern hemispheric upper troposphere (UT) and lowermost stratosphere (LMS). A large number of in-situ instruments were deployed on board a Learjet 35A, flying at altitudes up to 13.7 km, at times reaching to nearly 380 K potential temperature. Eight measurement campaigns (consisting of a total of 36 flights), distributed over all seasons and typically covering latitudes between 35 • N and 75 • N in the European longitude sector (10 • W-20 • E), were performed. Here we present an overview of the project, describing the instrumentation, the encountered meteorological situations during the campaigns and the data set available from SPURT. Measurements were obtained for N 2 O, CH 4 , CO, CO 2 , CFC12, H 2 , SF 6 , NO, NO y , O 3 and H 2 O. We illustrate the strength of this new data set by showing mean distributions of the mixing ratios of selected trace gases, using a potential temperature-equivalent latitude coordinate system. The observations reveal that the LMS is most stratospheric in character during spring, with the highest mixing ratios of O 3 and NO y and the lowest mixing ratios of N 2 O and SF 6 . The lowest mixing ratios of NO y and O 3 are observed during autumn, together with the highest mixing ratios of N 2 O and SF 6 indicating a strong tropospheric influence. For H 2 O, however, the maximum concentrations in the LMS are found during summer, suggesting unique (temperatureCorrespondence to: A. Engel (an.engel@meteor.uni-frankfurt.de) and convection-controlled) conditions for this molecule during transport across the tropopause. The SPURT data set is presently the most accurate and complete data set for many trace species in the LMS, and its main value is the simultaneous measurement of a suite of trace gases having different lifetimes and physical-chemical histories. It is thus very well suited for studies of atmospheric transport, for model validation, and for investigations of seasonal changes in the UT/LMS, as demonstrated in accompanying and elsewhere published studies.

No abstract

Abstract. Recent studies on the formation of a quasipermanent layer of enhanced static stability above the thermal tropopause revealed the contributions of dynamical and radiative processes. Dry dynamics leads to the evolution of a tropopause inversion layer (TIL), which is, however, too weak compared to observations and thus diabatic contributions are required. In this study we aim to assess the importance of diabatic processes in the understanding of TIL formation at midlatitudes. The non-hydrostatic model COSMO (COnsortium for Small-scale MOdelling) is applied in an idealized midlatitude channel configuration to simulate baroclinic life cycles. The effect of individual diabatic processes related to humidity, radiation, and turbulence is studied first to estimate the contribution of each of these processes to the TIL formation in addition to dry dynamics. In a second step these processes are stepwise included in the model to increase the complexity and finally estimate the relative importance of each process. The results suggest that including turbulence leads to a weaker TIL than in a dry reference simulation. In contrast, the TIL evolves stronger when radiation is included but the temporal evolution is still comparable to the reference. Using various cloud schemes in the model shows that latent heat release and consecutive increased vertical motions foster an earlier and stronger appearance of the TIL than in all other life cycles. Furthermore, updrafts moisten the upper troposphere and as such increase the radiative effect from water vapor. Particularly, this process becomes more relevant for maintaining the TIL during later stages of the life cycles. Increased convergence of the vertical wind induced by updrafts and by propagating inertia-gravity waves, which potentially dissipate, further contributes to the enhanced stability of the lower stratosphere. Finally, radiative feedback of ice clouds reaching up to the tropopause is identified to potentially further affect the strength of the TIL in the region of the clouds.