[1] The spread of mineral particles over southwestern, western, and central Europe resulting from a strong Saharan dust outbreak in October 2001 was observed at 10 stations of the European Aerosol Research Lidar Network (EARLINET). For the first time, an optically dense desert dust plume over Europe was characterized coherently with high vertical resolution on a continental scale. The main layer was located above the boundary layer (above 1-km height above sea level (asl)) up to 3-5-km height, and traces of dust particles reached heights of 7-8 km. The particle optical depth typically ranged from 0.1 to 0.5 above 1-km height asl at the wavelength of 532 nm, and maximum values close to 0.8 were found over northern Germany. The lidar observations are in qualitative agreement with values of optical depth derived from Total Ozone Mapping Spectrometer (TOMS) data. Ten-day backward trajectories clearly indicated the Sahara as the source region of the particles and revealed that the dust layer observed, e.g., over Belsk, Poland, crossed the EARLINET site Aberystwyth, UK, and southern Scandinavia 24-48 hours before. Lidar-derived particle depolarization ratios, backscatter-and extinction-related Å ngström exponents, and extinction-to-backscatter ratios mainly ranged from 15 to 25%, À0.5 to 0.5, and 40-80 sr, respectively, within the lofted dust plumes. A few atmospheric model calculations are presented showing the dust concentration over Europe. The simulations were found to be consistent with the network observations.
An intercomparison of the algorithms used to retrieve aerosol extinction and backscatter starting from Raman lidar signals has been performed by 11 groups of lidar scientists involved in the European Aerosol Research Lidar Network ͑EARLINET͒. This intercomparison is part of an extended quality assurance program performed on aerosol lidars in the EARLINET. Lidar instruments and aerosol backscatter algorithms were tested separately. The Raman lidar algorithms were tested by use of synthetic lidar data, simulated at 355, 532, 386, and 607 nm, with realistic experimental and atmospheric conditions taken into account. The intercomparison demonstrates that the data-handling procedures used by all the lidar groups provide satisfactory results. Extinction profiles show mean deviations from the correct solution within 10% in the planetary boundary layer ͑PBL͒, and backscatter profiles, retrieved by use of algorithms based on the combined Raman elastic-backscatter lidar technique, show mean deviations from solutions within 20% up to 2 km. The intercomparison was also carried out for the lidar ratio and produced profiles that show a mean deviation from the solution within 20% in the PBL. The mean value of this parameter was also calculated within a lofted aerosol layer at higher altitudes that is representative of typical layers related to special events such as Saharan dust outbreaks, forest fires, and volcanic eruptions. Here deviations were within 15%.
[1] During the Lindenberg Aerosol Characterization Experiment (LACE 98) simultaneous measurements with ground-based and airborne lidars and with two aircraft equipped with aerosol in situ instrumentation were performed. From the lidar measurements, particle backscatter coefficients at up to eight wavelengths between 320 and 1064 nm and particle extinction coefficients at 2-3 wavelengths between 292 and 532 nm were determined. Thus, for the first time, an extensive set of optical particle properties from several lidar platforms was available for the inversion into particle microphysical quantities. For this purpose, two different inversion algorithms were used, which provide particle effective radius, volume, surface-area, and number concentrations, and complex refractive index. The single-scattering albedo follows from Mie-scattering calculations. The parameters were compared to the ones from airborne measurements of particle size distributions and absorption coefficients. Two measurement cases were selected. During the night of 9 -10 August 1998 measurements were taken in a biomass-burning aerosol layer in the free troposphere, which was characterized by a particle optical depth of about 0.1 at 550 nm. Excellent agreement between remote-sensing and in situ measurements was found. In the center of this plume the effective radius was approximately 0.25 m, and all methods showed rather high complex refractive indices, ranging from 1.56 -1.66 in real part and from 0.05-0.07i in imaginary part. The single-scattering albedo showed low values from 0.78 -0.83 at 532 nm. The second case, taken on 11 August 1998, presents the typical conditions of a polluted boundary layer in central Europe. Optical depth was 0.35 at 550 nm, and particle effective radii were 0.1-0.2 m. In contrast to the first case, imaginary parts of the refractive index were below 0.03i. Accordingly, the single-scattering albedo ranged from 0.87-0.95.
The vertical allocation of emissions has a major impact on results of Chemistry Transport Models. However, in Europe it is still common to use fixed vertical profiles based on rough estimates to determine the emission height of point sources. This publication introduces a set of new vertical profiles for the use in chemistry transport modeling that were created from hourly gridded emissions calculated by the SMOKE for Europe emission model. SMOKE uses plume rise calculations to determine effective emission heights. Out of more than 40 000 different vertical emission profiles 73 have been chosen by means of hierarchical cluster analysis. These profiles show large differences to those currently used in many emission models. Emissions from combustion processes are released in much lower altitudes while those from production processes are allocated to higher altitudes. The profiles have a high temporal and spatial variability which is not represented by currently used profiles.
[1] Since 2000, regular lidar observations of the vertical aerosol distribution over Europe have been performed within the framework of EARLINET, the European Aerosol Research Lidar Network. A statistical analysis concerning the vertical distribution of the volume light extinction coefficients of particles derived from Raman lidar measurements at 10 EARLINET stations is presented here. The profiles were measured on a fixed schedule with up to two measurements per week; they typically covered the height range from 500 m to 6000 m above ground level (agl). The analysis is made for the planetary boundary layer (PBL) as well as for several fixed layers above ground. The results show typical values of the aerosol extinction coefficient and the aerosol optical depth (AOD) in different parts of Europe, with highest values in southeastern Europe and lowest values in the northwestern part. Annual cycles and cumulative frequency distributions are also presented. We found that higher aerosol optical depths in southern Europe compared to the northern part are mainly attributed to larger amounts of aerosol in higher altitudes. At 9 of the 10 sites the frequency distribution of the aerosol optical depth in the planetary boundary layer follows a lognormal distribution at the 95% significance level.
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