Proportional electroluminescence (EL) in noble gases has long been used in two-phase detectors for dark matter search, to record ionization signals induced by particle scattering in the noble-gas liquid (S2 signals). Until recently, it was believed that proportional electroluminescence was fully due to VUV emission of noble gas excimers produced in atomic collisions with excited atoms, the latter being in turn produced by drifting electrons. In this work we consider an additional mechanism of proportional electroluminescence, namely that of bremsstrahlung of drifting electrons scattered on neutral atoms (so-called neutral bremsstrahlung); it is systemically studied here both theoretically and experimentally. In particular, the absolute EL yield has for the first time been measured in pure gaseous argon in the two-phase mode, using a dedicated two-phase detector with EL gap optically read out by cryogenic PMTs and SiPMs. We show that the neutral bremsstrahlung effect can explain two intriguing observations in EL radiation: that of the substantial contribution of the non-VUV spectral component, extending from the UV to NIR, and that of the photon emission at lower electric fields, below the Ar excitation threshold. Possible applications of neutral bremsstrahlung effect in two-phase dark matter detectors are discussed.
PACS 95.55.Vj -Neutrino, muon,pion, and other elementary particle detectors; cosmic ray detectors PACS 61.25.Bi -Liquid noble gases PACS 95.35.+d -Dark matter Abstract -Proportional electroluminescence (EL) in gaseous Ar has for the first time been systematically studied in the two-phase mode, at 87 K and 1.00 atm. Liquid argon had a minor (56 ppm) admixture of nitrogen, which allowed to understand, inter alia, the effect of N2 doping on the EL mechanism in rare-event experiments using two-phase Ar detectors. The measurements were performed in a two-phase Cryogenic Avalanche Detector (CRAD) with EL gap located directly above the liquid-gas interface. The EL gap was optically read out in the Vacuum Ultraviolet (VUV), near 128 nm (Ar excimer emission), and in the near Ultraviolet (UV), at 300-450 nm (N2 Second Positive System emission), via cryogenic PMTs and a Geiger-mode APD (GAPD). Proportional electroluminescence was measured to have an amplification parameter of 109±10 photons per drifting electron per kV overall in the VUV and UV, of which 51±6% were emitted in the UV. The measured EL threshold, at an electric field of 3.7±0.2 kV/cm, was in accordance with that predicted by the theory. The latter result is particularly relevant to DarkSide and SCENE dark matter search-related experiments, where the operation electric field was thereby on the verge of appearance of the S2 (ionization-induced) signal. The results obtained pave the way to the development of N2-doped two-phase Ar detectors with enhanced sensitivity to the S2 signal.(a) Corresponding author. Email: A.F.Buzulutskov@inp.nsk.su emitted from the liquid, drift in a moderate electric field in an electroluminescence (EL) gap located directly above the liquid-gas interface. In proportional electroluminescence the photon yield is basically proportional to the electric field, since the energy provided to the electrons by the electric field is almost fully expended in atomic excitations producing Ar * (3p 5 4s 1 ) and Ar * (3p 5 4p 1 ) states (the first one being metastable). These are followed by the photon emission in the Vacuum Ultraviolet (VUV), around 128 nm, due to excimer productions in three-body collisions and their subsequent decays [11][12][13] Ar * (3p 5 4s 1 ) + 2Ar → Ar * 2 + Ar, Ar * 2 → 2Ar + hν, (1) and by the photon emission in the Near Infrared (NIR), at 690-850 nm, due to Ar * (3p 5 4p 1 ) → Ar * (3p 5 4s 1 ) + hν atomic transitions [14][15][16].
We further study the effect of neutral bremsstrahlung (NBrS) in two-phase argon electroluminescence (EL), revealed recently in [1]. The absolute EL yield due to NBrS effect, in the visible and NIR range, was remeasured in pure gaseous argon in the two-phase mode, using a two-phase detector with EL gap read out directly by cryogenic PMTs and SiPMs. Possible applications of the NBrS effect in detection science are discussed, including those in two-phase dark matter detectors.
A two-phase Cryogenic Avalanche Detector (CRAD) with electroluminescence (EL) gap, operated in argon doped with a minor (49±7 ppm) admixture of nitrogen, has been studied. The EL gap was optically read out using cryogenic PMTs located on the perimeter of the gap. We present the results of the measurements of the N 2 content, detector sensitivity to X-ray-induced signals, EL gap yield and electron lifetime in the liquid. The detector sensitivity, at a drift field in liquid Ar of 0.6 kV/cm, was measured to be 9 and 16 photoelectrons recorded at the PMTs per keV of deposited energy at 23 and 88 keV respectively. Such two-phase detectors, with enhanced sensitivity to the S2 (ionization-induced) signal, are relevant in the field of argon detectors for dark matter search and low energy neutrino detection.
Proportional electroluminescence (EL) in noble gases is used in two-phase detectors for dark matter searches to record (in the gas phase) the ionization signal induced by particle scattering in the liquid phase. The “standard” EL mechanism is considered to be due to noble gas excimer emission in the vacuum ultraviolet (VUV). In addition, there are two alternative mechanisms, producing light in the visible and near infrared (NIR) ranges. The first is due to bremsstrahlung of electrons scattered on neutral atoms (“neutral bremsstrahlung”, NBrS). The second, responsible for electron avalanche scintillation in the NIR at higher electric fields, is due to transitions between excited atomic states. In this work, we have for the first time demonstrated two alternative techniques of the optical readout of two-phase argon detectors, in the visible and NIR range, using a silicon photomultiplier matrix and electroluminescence due to either neutral bremsstrahlung or avalanche scintillation. The amplitude yield and position resolution were measured for these readout techniques, which allowed to assess the detection threshold for electron and nuclear recoils in two-phase argon detectors for dark matter searches. To the best of our knowledge, this is the first practical application of the NBrS effect in detection science.
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