This work presents for the first time, a simple, practical and scalable approach to fabricating recycled polyethylene terephthalate (rPET) aerogels for thermal and acoustic insulation applications. The rPET aerogels were successfully developed from recycled PET fibers and polyvinyl alcohol (PVA) and glutaraldehyde (GA) cross-linkers using a freeze-drying process. The effects of various PET fiber concentrations (0.5, 1.0 and 2.0 by wt.%), fiber deniers (3D, 7D and 15D) and fiber lengths (32 mm and 64 mm) on the rPET aerogel structures and multi-properties were comprehensively investigated. The developed rPET aerogels showed a highly porous network structure (98.3–99.5%), ultra-low densities (0.007–0.026 g/cm3), hydrophobicity with water contact angles of 120.7–149.8°, and high elasticity with low compressive Young’s modulus (1.16–2.87 kPa). They exhibited superior thermal insulation capability with low thermal conductivities of 0.035–0.038 W/m.K, which are highly competitive with recycled cellulose and silica-cellulose aerogels and better than mineral wool and polystyrene. The acoustic absorption results were also found to outperform a commercial acoustic foam absorber across a range of frequencies.
This work investigates the effects of interlayer hybrid fiber dispersion on the impact response of carbon-flax epoxy hybrid laminates at low carbon volume fractions, and benchmarks the mechanical performance enhancement against the non-hybrid flax epoxy. Five hybrid laminate stacking sequences with similar carbon-to-flax weight ratio were fabricated and subjected to low-velocity impact at three different energy values, generating non-perforated and perforated damage states. A virtual drop-weight impact test that models intralaminar failure based on continuum damage mechanics approach, and delamination using cohesive elements, was also implemented to evaluate the material behavior and damage development in the composites. Simulation results were then verified against experimental data. Results suggested that positioning stiffer carbon plies at the impact face does not necessarily lead to enhancement of the hybrid's impact properties. On the contrary, flax plies at the impacted side lead to significant improvement in impact resistance compared to the non-hybrid flax composite with similar thickness. Results of finite element analysis showed that carbon plies play a significant role in the hybrid laminate's energy absorption characteristics due to lower failure strain.
Natural fibers and their composites differ in several aspects with carbon fibers, including higher scatter in strength and different tensile responses. The tensile and bending properties of flax fiber composites were experimentally studied and numerically simulated. Composite panels were fabricated from unidirectional flax fiber tapes and polypropylene films via hot pressing technique. The variation in the properties of flax/polypropylene composites was found to be relatively moderate as compared with that of single natural fibers. A multi-scale finite element analysis (FEA) strategy for the progressive damage prediction of natural fiber composites was developed. The FEA model started from microscale analysis which predicted the effective properties of unidirectional flax ply through representative volume element. Macro-scale analysis was conducted subsequently to predict the properties of composite coupons using the results of micro-scale analysis as inputs. The developed multi-scale FE model successfully predicted the tensile strength, bending behavior, and major failure modes of flax/polypropylene composites.
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