The measurement of the Cu-O distances by a local and fast probe, polarized Cu K-edge extended x-ray absorption fine structure (EXAFS) in La 1.85 Sr 0.15 CuO 4 crystal shows two different conformations of the CuO 6 octahedra below 100 K assigned to two types of stripes with different lattice. This experiment supports a model of "two components" spatially separated in a superlattice of quantum stripes for the anomalous properties of cuprate superconductors. [S0031-9007(96)00119-6] PACS numbers: 74.72. Dn, 61.10.Ht, 78.70.Dm Experimental methods probing the local structure have shown that the structure of the metallic CuO 2 plane in high T c cuprate superconductors is not homogeneous at a mesoscopic scale length [1][2][3][4]. It has been proposed that an anharmonic 1D modulation of the CuO 2 plane is a key feature for the mechanism of high T c superconductivity [5]. A superstructure of the type q pb ء 1 ͑1͞n͒c ء , in the orthorhombic notation, seems to be a common feature of the superconducting cuprates close to the optimum doping. It has been observed in Bi 2 Sr 2 CaCu 2 O 81d (Bi2212) [6,7] and in Bi 2 Sr 2 Cu 2 O 61d (Bi2201) [8] with p ϳ 0.21 and n 2 considering doubling of the c axis; in La 2 CuO 4.1 (LCO) with p 0.22 and n 3 [9] and with p 0.2 and n 3 [10]; in La 22x Sr x Cu 2 O 4 (LSCO) for x ϳ 0.075 with p ϳ 0.16 and n ϳ 2.5 [11] and a similar superstructure for x 0.1, 0.15 but much weaker in intensity for the overdoped sample, i.e., x 0.2 [12]; in Tl 2 Ba 2 CaCu 2 O 8 (Tl2212) with p ϳ 0.2 [13] and a similar one in Tl 2 Ba 2 Ca 2 Cu 3 O 10 (Tl2223) [14]. This superstructure is difficult to identify in some of the compounds (for example, in the case of LSCO it could be identified only after about 9 yr of the discovery of high T c superconductivity in this material), and it is more clear at temperatures lower than 100-200 K (e.g., in Tl2212, Tl2223, LCO, LSCO). On the other hand, the superstructure is stable even at high temperatures in Bi2212. The c-axis modulation, different from sample to sample, is due to ordering of dopants in the rock-salt block layers as it is clear in the isostructural compounds, e.g., La 2 NiO 41d . The long wavelength incommensurate modulation of the CuO 2 plane along the 45 ± direction from the Cu-Cu direction, involving ϳ10 Cu sites, appears to be a common feature of cuprate superconductors at optimum doping.A "two-component" model has been proposed [5] where at optimum doping (0.2 hole per Cu sites) a first component with hole density d i ϳ 1 1 0.16 coexists with a second component of impurity states, with hole density d ᐉ ϳ 0.04, spatially separated in two different types of stripes forming a superlattice of quantum wires. A com-mensurate superstructure with lower period (4 Cu sites) was predicted [5] where all doped holes form a single electronic component, a pinned Wigner polaronic charge density wave (CDW), that will suppress superconductivity, and it has been observed at the 1͞8 critical doping and in the nickelates [15].In the case of Bi2212 we have shown [5] that th...
An ordered phase showing remarkable electronic anisotropy in proximity to the superconducting phase is now a hot issue in the field of high-transition-temperature superconductivity. As in the case of copper oxides, superconductivity in iron arsenides competes or coexists with such an ordered phase. Undoped and underdoped iron arsenides have a magnetostructural ordered phase exhibiting stripe-like antiferromagnetic spin order accompanied by an orthorhombic lattice distortion; both the spin order and lattice distortion break the tetragonal symmetry of crystals of these compounds. In this ordered state, anisotropy of in-plane electrical resistivity is anomalous and difficult to attribute simply to the spin order and/or the lattice distortion. Here, we present the anisotropic optical spectra measured on detwinned BaFe 2 As 2 crystals with light polarization parallel to the Fe planes. Pronounced anisotropy is observed in the spectra, persisting up to an unexpectedly high photon energy of about 2 eV. Such anisotropy arises from an anisotropic energy gap opening below and slightly above the onset of the order. Detailed analysis of the optical spectra reveals an unprecedented electronic state in the ordered phase.anisotropic electronic state | iron pnictide | optical spectrum H igh-transition-temperature (high-T c ) superconductivity realized in both copper oxides and iron arsenides shares common features, namely, the superconducting phase is in close proximity to a symmetry-breaking phase and these phases coexist under certain circumstances, but apparently compete with each other. The close proximity suggests that our understanding of high-T c superconductivity will greatly improve once the nature of this proximate phase is revealed. The parent compounds of iron-arsenide superconductors, with BaFe 2 As 2 as a representative example, are unique metals that undergo a tetragonal-toorthorhombic structural phase transition at temperature T s with a shorter b axis and a longer a axis in the orthorhombic phase always accompanied by antiferromagnetic (AF) spin order at temperature T N . T N is equal to T s in some compounds (1-3) and slightly lower than T s in others (4). BaFe 2 As 2 exhibits stripe-like AF order in which Fe spins align antiferromagnetically in the a-axis direction in the Fe plane and ferromagnetically in the b-axis direction. Anisotropic electronic properties have been experimentally examined by various methods, such as neutron scattering (5), scanning tunneling microscopy (STM) (6), and angleresolved photoemission spectroscopy (ARPES) (7,8). These experiments suggest strong anisotropy of spin excitation and of the shape of Fermi surfaces. However, most of the experiments were performed on twinned crystals with randomly oriented domains, which inhibit the observation of genuine anisotropy.Recently, anisotropic resistivity has been measured on detwinned crystals (9, 10). The anisotropy of resistivity is quite anomalous in that the resistivity along the spin-ferromagnetic (FM) direction with a shorter b axis is...
We report muon spin relaxation (SR) measurements using single crystals of oxygen-intercalated stage-4 La 2 CuO 4.11 ͑LCO:4.11͒ and La 1.88 Sr 0.12 CuO 4 ͑LSCO:0.12͒, in which neutron scattering studies have found incommensurate magnetic Bragg reflections. In both systems, zero-field SR measurements show muon spin precession below the Néel temperature T N with frequency 3.6 MHz at T→0, having a Bessel function line shape, characteristic of spin-density-wave systems. The amplitude of the oscillating and relaxing signals of these systems is less than half the value expected for systems with static magnetic order in 100% of the volume. Our results are consistent with a simulation of local fields for a heuristic model with ͑a͒ incommensurate spin amplitude modulation with the maximum ordered Cu moment size of ϳ0.36 B , ͑b͒ static Cu moments on the CuO 2 planes forming ''islands'' having typical radius 15-30 Å, comparable to the in-plane superconducting coherence length, and ͑c͒ the measured volume fraction of magnetic muon sites V increasing progressively with decreasing temperature below T N towards V ϳ40% for LCO:4.11 and 18% for LSCO:0.12 at T→0. These results may be compared with correlation lengths in excess of 600 Å and a long range ordered moment of 0.15Ϯ0.05 B measured with neutron scattering techniques. In this paper we discuss a model that reconciles these apparently contradictory results. In transverse magnetic field SR measurements, sensitive to the in-plane magnetic field penetration depth ab , the results for LCO:4.11 and LSCO:0.12 follow correlations found for underdoped, overdoped and Zn-doped high-T c cuprate systems in a plot of T c versus the superconducting relaxation rate (T→0). This indicates that the volume-integrated value of n s /m* ͑superconducting carrier density / effective mass͒ is a determining factor for T c , not only in high-T c cuprate systems without static magnetism, but also in the present systems where superconductivity coexists with static spin-densitywave spin order.
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