A novel approach to mass measurements at the 10−9 level for short-lived nuclides with half-lives well below one second is presented. It is based on the projection of the radial ion motion in a Penning trap onto a position-sensitive detector. Compared with the presently employed time-of-flight ion-cyclotron-resonance technique, the novel approach is 25-times faster and provides a 40-fold gain in resolving power. Moreover, it offers a substantially higher sensitivity since just two ions are sufficient to determine the ion’s cyclotron frequency. Systematic effects specific to the technique that can change the measured cyclotron frequency are considered in detail. It is shown that the main factors that limit the maximal accuracy and resolving power of the technique are collisions of the stored ions with residual gas in the trap, the temporal instability of the trapping voltage, the anharmonicities of the trapping potential and the uncertainty introduced by the conversion of the cyclotron to magnetron motion
The Phase-Imaging Ion-Cyclotron-Resonance (PI-ICR) technique has been commissioned at the JYFLTRAP double Penning trap mass spectrometer. This technique is based on projecting the ion motion in the Penning trap onto a position-sensitive multichannel-plate ion detector. Mass measurements of stable 85 Rb + and 87 Rb + ions with well-known mass values show that relative uncertainties ∆m/m ≤ 7 · 10 −10 are possible to reach with the PI-ICR technique at JYFLTRAP. The significant improvement both in resolving power and in precision compared to the conventional Time-of-Flight Ion Cyclotron Resonance technique will enable measurements of close-lying isomeric states and of more exotic isotopes as well as ultra-high precision measurements required, e.g., for neutrino physics. In addition, a new phase-dependent cleaning method based on the differences in the accumulated cyclotron motion phases has been demonstrated with short-lived 127 In + and 127m In + ions.
In this article a comprehensive description and performance of the double Penning trap setup JYFLTRAP will be detailed. The setup is designed for atomic mass measurements of both radioactive and stable ions and additionally serves as a very high resolution mass separator. The setup is coupled to the IGISOL facility at the accelerator laboratory of the University of Jyväskylä. The trap has been online since 2003 and it was shut down in summer 2010 for relocation to upgraded IGISOL facility. Numerous atomic mass and decay energy measurements have been performed using the time-of-flight ion-cyclotron resonance technique. Also the trap has been used in several decay spectroscopy experiments as a high-resolution mass filter.
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