We study the transport properties of the Kondo insulator SmB 6 with a specialized configuration designed to distinguish bulk-dominated conduction from surface-dominated conduction. We find that as the material is cooled below 4 K, it exhibits a crossover from bulk to surface conduction with a fully insulating bulk. We take the robustness and magnitude of the surface conductivity, as is manifest in the literature of SmB 6 , to be strong evidence for the topological insulator metallic surface states recently predicted for this material.
In Kondo insulator samarium hexaboride SmB6, strong correlation and band hybridization lead to an insulating gap and a diverging resistance at low temperature. The resistance divergence ends at about 5 Kelvin, a behavior recently demonstrated to arise from the surface conductance. However, questions remain whether and where a topological surface state exists. Quantum oscillations have not been observed to map the Fermi surface. We solve the problem by resolving the Landau Level quantization and Fermi surface topology using torque magnetometry. The observed Fermi surface suggests a two dimensional surface state on the (101) plane. Furthermore, the tracking of the Landau Levels in the infinite magnetic field limit points to -1/2, which indicates a 2D Dirac electronic state.The recent development of topological insulators is a triumph of single electron band theory [1][2][3][4][5][6][7][8] . It is interesting to understand whether similar exotic states of matter can arise once strong electronic interaction comes into play. Kondo insulators, a strongly-correlated heavyfermion system, offer a good playground for the exploration of this question. In a Kondo insulator 9,10 , the hybridization between itinerant electrons and localized orbitals opens a gap and makes the material insulating. Once the sample temperature is cold enough, the electronic structure in the strongly correlated system can be mapped to a rather simple electronic state that resembles a normal topological insulator 11 . As a result, in the ground state of the Kondo insulator there exists a bulk insulating state and a conductive surface state. In samarium hexaboride (SmB 6 ), the existence of the surface state has been suggested by recent experimental observations of the surface conductance as well as a map of the hybridization gap 12-14 . However, a direct observation of the Fermi surface has not yet been achieved by transport measurements in Kondo insulators. In this letter we report the observation of quantum oscillations in Kondo insulator SmB 6 using torque magnetometry. The observed Fermi surface is shown to be two-dimensional (2D) and arises from the crystalline (101) surface, and the Landau Level index plot shows a Berry phase contributed -1/2 factor in the infinite field limit, which indicates that this Fermi surface encloses Dirac points, a characteristic property of topological insulators.The direct observation of quantum oscillations is an essential step in understanding the electronic state of the bulk and surfaces of Kondo insulator. Wolgast et al. have argued strongly that the great robustness and certain other properties of the low T surface conductivity of SmB 6 are best understood as a consequence of having TI surface states 12 . Nonetheless there is yet no direct evidence for this interpretation of the surface conduction. Such evidence should come from microscopic measurements of the electronic structure, as has been accomplished for the weakly correlated TI materials, such as Bi 2 Se 3 , Bi 2 Te 3 , and graphene [15][16][17][18][19...
The recent conjecture of a topologically-protected surface state in SmB 6 and the verification of robust surface conduction below 4 K have prompted a large effort to understand the surface states.Conventional Hall transport measurements allow current to flow on all surfaces of a topological insulator, so such measurements are influenced by contributions from multiple surfaces of varying transport character. Instead, we study magnetotransport of SmB 6 using a Corbino geometry, which can directly measure the conductivity of a single, independent surface. Both (011) and (001) crystal surfaces show a strong negative magnetoresistance at all magnetic field angles measured.The (011) surface has a carrier mobility of 122 cm 2 /V·sec with a carrier density of 2.5×10 13 cm −2 , which are significantly smaller than indicated by Hall transport studies. This mobility value can explain a failure so far to observe Shubnikov-de Haas oscillations. Analysis of the angle-dependence of conductivity on the (011) surface suggests a combination of a field-dependent enhancement of the carrier density and a suppression of Kondo scattering from native oxide layer magnetic moments as the likely origin of the negative magnetoresistance. Our results also reveal a hysteretic behavior whose magnitude depends on the magnetic field sweep rate and temperature. Although this feature becomes smaller when the field sweep is slower, does not disappear or saturate during our slowest sweep-rate measurements, which is much slower than a typical magnetotransport trace.These observations cannot be explained by quantum interference corrections such as weak antilocalization, but are more likely due to an extrinsic magnetic effect such as the magnetocaloric effect or glassy ordering.
After the theoretical prediction that SmB6 is a topological Kondo insulator, there has been an explosion of studies on the SmB6 surface. However, there is not yet an agreement on even the most basic quantities such as the surface carrier density and mobility. In this paper, we carefully revisit Corbino disk magnetotransport studies to find those surface transport parameters. We first show that subsurface cracks exist in the SmB6 crystals, arising both from surface preparation and during the crystal growth. We provide evidence that these hidden subsurface cracks are additional conduction channels, and the large disagreement between earlier surface SmB6 studies may originate from previous interpretations not taking this extra conduction path into account. We provide an update of a more reliable magnetotransport data than the previous one (Phys. Rev. B 92, 115110) and find that the orders-of-magnitude large disagreements in carrier density and mobility come from the surface preparation and the transport geometry rather than the intrinsic sample quality. From this magnetotransport study, we find an updated estimate of the carrier density and mobility of 2.71×10 13 (1/cm 2 ) and 104.5 (cm 2 /V·sec), respectively. We compare our results with other studies of the SmB6 surface. By this comparison, we provide insight into the disagreements and agreements of the previously reported angle-resolved photoemission spectroscopy, scanning tunneling microscopy, and magnetotorque quantum oscillations measurements.
SmB 6 exhibits a small (15-20 meV) bandgap at low temperatures due to hybridized d and f electrons, a tiny (3 meV) transport activation energy (E A ) above 4 K, and surface states accessible to transport below 2 K. We study its magnetoresistance in 60-T pulsed fields between 1.5 K and 4 K. The response of the nearly T -independent surface states (which show no Shubnikov-de Haas oscillations) is distinct from that of the activated bulk. E A shrinks by 50% under fields up to 60 T. Data up to 93 T suggest that this trend continues beyond 100 T, in contrast with previous explanations. It rules out emerging theories to explain observed exotic magnetic quantum oscillations.
In an ideal topological insulator, the helical spin structure of surface electrons suppresses backscattering and thus can enhance surface conductivity. In this study, we investigate the effect of perpendicular magnetic field on the spin structure of electrons at the Fermi energy and define a magnetic-field dependent topological enhancement factor using Boltzmann transport and calculate this factor for different disorder potentials, ranging from short-range disorder to screened Coulomb potential. Within the Boltzmann approximation, the topological enhancement factor reaches its maximum value of 4 for a short-range disorder at zero magnetic field and approaches a value of 1 at high magnetic fields. The topological enhancement factor becomes independent of the nature of the disorder potential at high magnetic fields.
Abstract:We report on a strong effect of p-GaN surface morphology on the growth mode and surface roughness of ZnO:Ga films grown by plasma-assisted molecular-beam epitaxy on p-GaN/c-sapphire templates. A range of ZnO:Ga surface morphologies varying from rough surfaces with well defined three-dimensional islands, capable to enhance light extraction in light-emitting diodes, to rather smooth surfaces with a surface roughness of ~ 2 nm suitable for vertical-cavity lasers can be achieved by controlling the surface morphologies of p-GaN. Optical transmittance measurements revealed high transparency exceeding 90% in the visible spectral range for ZnO:Ga with both types of surface morphology.
Measuring the temperature profile of a nanoscale sample using scanning thermal microscopy is challenging due to a scanning probe's non-uniform heating. In order to address this challenge, we have developed a calibration sample consisting of a 1-lm wide gold wire, which can be heated electrically by a small bias current. The Joule heating in the calibration sample wire is characterized using noise thermometry. A thermal probe was scanned in contact over the gold wire and measured temperature changes as small as 0.4 K, corresponding to 17 ppm changes in probe resistance. The non-uniformity of the probe's temperature profile during a typical scan necessitated the introduction of a temperature conversion factor, g, which is defined as the ratio of the average temperature change of the probe with respect to the temperature change of the substrate. The conversion factor was calculated to be 0.035 6 0.007. Finite element analysis simulations indicate a strong correlation between thermal probe sensitivity and probe tip curvature, suggesting that the sensitivity of the thermal probe can be improved by increasing the probe tip curvature, though at the expense of the spatial resolution provided by sharper tips. Simulations also indicate that a bow-tie metallization design could yield an additional 5-to 7-fold increase in sensitivity.
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