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[1] Using NASA's A-Train satellite measurements, we evaluate the accuracy of cloud water content (CWC) and water vapor mixing ratio (H 2 O) outputs from 19 climate models submitted to the Phase 5 of Coupled Model Intercomparison Project (CMIP5), and assess improvements relative to their counterparts for the earlier CMIP3. We find more than half of the models show improvements from CMIP3 to CMIP5 in simulating column-integrated cloud amount, while changes in water vapor simulation are insignificant. For the 19 CMIP5 models, the model spreads and their differences from the observations are larger in the upper troposphere (UT) than in the lower or middle troposphere (L/MT). The modeled mean CWCs over tropical oceans range from $3% to $15Â of the observations in the UT and 40% to 2Â of the observations in the L/MT. For modeled H 2 Os, the mean values over tropical oceans range from $1% to 2Â of the observations in the UT and within 10% of the observations in the L/MT. The spatial distributions of clouds at 215 hPa are relatively well-correlated with observations, noticeably better than those for the L/MT clouds. Although both water vapor and clouds are better simulated in the L/MT than in the UT, there is no apparent correlation between the model biases in clouds and water vapor. Numerical scores are used to compare different model performances in regards to spatial mean, variance and distribution of CWC and H 2 O over tropical oceans. Model performances at each pressure level are ranked according to the average of all the relevant scores for that level.Citation: Jiang, J. H., et al. (2012), Evaluation of cloud and water vapor simulations in CMIP5 climate models using NASA "A-Train" satellite observations,

Abstract. We use a coupled atmosphere-ocean global climate model (CSIRO-Mk3.6) to investigate the drivers of trends in summer rainfall and circulation in the vicinity of northern Australia. As part of the Coupled Model Intercomparison Project Phase 5 (CMIP5), we perform a 10-member 21st century ensemble driven by Representative Concentration Pathway 4.5 (RCP4.5). To investigate the roles of different forcing agents, we also perform multiple 10-member ensembles of historical climate change, which are analysed for the period 1951–2010. The historical runs include ensembles driven by "all forcings" (HIST), all forcings except anthropogenic aerosols (NO_AA) and forcing only from long-lived greenhouse gases (GHGAS). Anthropogenic aerosol-induced effects in a warming climate are calculated from the difference of HIST minus NO_AA. CSIRO-Mk3.6 simulates a strong summer rainfall decrease over north-western Australia (NWA) in RCP4.5, whereas simulated trends in HIST are weakly positive (but insignificant) during 1951–2010. The weak rainfall trends in HIST are due to compensating effects of different forcing agents: there is a significant decrease in GHGAS, offset by an aerosol-induced increase. Observations show a significant increase of summer rainfall over NWA during the last few decades. The large magnitude of the observed NWA rainfall trend is not captured by 440 unforced 60-yr trends calculated from a 500-yr pre-industrial control run, even though the model's decadal variability appears to be realistic. This suggests that the observed trend includes a forced component, despite the fact that the model does not simulate the magnitude of the observed rainfall increase in response to "all forcings" (HIST). We investigate the mechanism of simulated and observed NWA rainfall changes by exploring changes in circulation over the Indo-Pacific region. The key circulation feature associated with the rainfall increase in reanalyses is a lower-tropospheric cyclonic circulation trend off the coast of NWA, which enhances the monsoonal flow. The model shows an aerosol-induced cyclonic circulation trend off the coast of NWA in HIST minus NO_AA, whereas GHGAS shows an anticyclonic circulation trend. This explains why the aerosol-induced effect is an increase of rainfall over NWA, and the greenhouse gas-induced effect is of opposite sign. Possible explanations for the cyclonic (anticyclonic) circulation trend in HIST minus NO_AA (GHGAS) involve changes in the Walker circulation or the local Hadley circulation. In either case, a plausible atmospheric mechanism is that the circulation anomaly is a Rossby wave response to convective heating anomalies south of the Equator. We also discuss the possible role of air-sea interactions, e.g. an increase (decrease) of sea-surface temperatures off the coast of NWA in HIST minus NO_AA (GHGAS). Further research is needed to better understand the mechanisms and the extent to which these are model-dependent. In summary, our results suggest that anthropogenic aerosols may have "masked" greenhouse gas-induced changes in rainfall over NWA and in circulation over the wider Indo-Pacific region. Due to the opposing effects of greenhouse gases and anthropogenic aerosols, future trends may be very different from trends observed over the last few decades.

[1] The vertical distributions of cloud water content (CWC) and cloud fraction (CF) over the tropical oceans, produced by 13 coupled atmosphere-ocean models submitted to the Phase 5 of Coupled Model Intercomparison Project (CMIP5), are evaluated against CloudSat/CALIPSO observations as a function of large-scale parameters. Available CALIPSO simulator CF outputs are also examined. A diagnostic framework is developed to decompose the cloud simulation errors into large-scale errors, cloud parameterization errors and covariation errors. We find that the cloud parameterization errors contribute predominantly to the total errors for all models. The errors associated with large-scale temperature and moisture structures are relatively greater than those associated with large-scale midtropospheric vertical velocity and lower-level divergence. All models capture the separation of deep and shallow clouds in distinct large-scale regimes; however, the vertical structures of high/low clouds and their variations with large-scale parameters differ significantly from the observations. The CWCs associated with deep convective clouds simulated in most models do not reach as high in altitude as observed, and their magnitudes are generally weaker than CloudSat total CWC, which includes the contribution of precipitating condensates, but are close to CloudSat nonprecipitating CWC. All models reproduce maximum CF associated with convective detrainment, but CALIPSO simulator CFs generally agree better with CloudSat/CALIPSO combined retrieval than the model CFs, especially in the midtroposphere. Model simulated low clouds tend to have little variation with large-scale parameters except lower-troposphere stability, while the observed low cloud CWC, CF, and cloud top height vary consistently in all large-scale regimes. Citation: Su, H., et al. (2013), Diagnosis of regime-dependent cloud simulation errors in CMIP5 models using "A-Train" satellite observations and reanalysis data,

The application of the Nesbet algorithm to the full iterative solution of the two-dimensional master equation for thermal unimolecular reactions is presented. This leads to an efficient algorithm for computing thermal rate coefficients in the falloff regime for reactions such as simple fission dissociations, radical-radical recombinations, and ion-molecule reactions wherein microcanonical dissociation rate coefficients are sensitive to both the vibrational energy and the angular momentum of the excited species.