Ultrathin emissive layers (UEMLs) of phosphorescent materials with a layer thickness of less than 0.3 nm were introduced for high-efficiency organic light-emitting diodes (OLEDs). All the UEMLs for white OLEDs can be prepared without the use of interlayers or spacers. Compared with devices fabricated with interlayers inserted in-between the UEMLs, our spacer-free structure not only significantly improves device efficiency, but also simplifies the fabrication process, thus it has a great potential in lowering the cost of OLED panels. In addition, its spacer-free structure decreases the number of interfaces which often introduce unnecessary energy barriers in these devices. In the present work, UEMLs of red, green and blue-emitting phosphorescent materials and yellow and blue phosphorescent emitters are utilized for the demonstration of spacer-free white OLEDs. Upon optimization of the device structure, we demonstrated spacer-free and simple-structured white-emitting OLEDs with a good device performance. The current and power efficiencies of our white-emitting devices are as high as 56.0 cd/A and 55.5 lm/W, respectively. These efficiencies are the highest ever reported for OLEDs fabricated with the UEML approach.
The bone defects caused by trauma are inevitably accompanied
by
soft tissue damage. The development of multifunctional bioactive biomaterials
with integrated bone and soft tissue regeneration is necessary and
needed urgently in orthopedics. In this work, we found that the photoactivated
MXene (Ti3C2T
x
)
nanosheet showed positive effects on promoting both bone and soft
tissue regeneration. We further investigated the detailed effect and
potential mechanism of photoactivated MXene on tissue regeneration.
Photoactivated MXene shows a good thermal effect and robust antibacterial
activity to inhibit the expression of inflammation factors and methicillin-resistant Staphylococcus aureus (MRSA) infection and induces the expression
of pro-angiogenic factors and soft tissue wound repair. Photoactivated
MXene can also regulate the osteogenic differentiation of adipose-derived
stem cells (ADSCs) through the ERK signaling pathway by activating
the heat shock protein 70 (HSP70) and enhancing the repair of bone
tissue. This work sheds light on the development of bioactive MXene
with photothermal activation as an efficient strategy for bone and
soft tissue regeneration simultaneously.
Magnetic skyrmions are topologically non-trivial spin structure, and their existence in ferromagnetically coupled multilayers has been reported with disordered arrangement. In these multilayers, the heavy metal spacing layers provide an interfacial Dzyaloshinskii-Moriya interaction (DMI) for stabilizing skyrmions at the expense of interlayer exchanging coupling (IEC). To meet the functional requirement of ordered/designable arrangement, in this work, we proposed and experimentally demonstrated a scenario of skyrmion nucleation using nanostructured synthetic antiferromagnetic (SAF) multilayers. Instead of relying on DMI, the antiferromagnetic IEC in the SAF multilayers fulfills the role of nucleation and stabilization of skyrmions. The IEC induced skyrmions were identified directly imaged with MFM and confirmed by magnetometry and magnetoresistance measurements as well as micromagnetic simulation. Furthermore, the robustness of the proposed skyrmion nucleation scenario was examined against temperature (from 4.5 to 300 K), device size (from 400 to 1200 nm), and different lattice designs. Hence, our results provide a synthetic skyrmion platform meeting the functional needs in magnonic and spintronic applications.
Spin-orbit torque (SOT) induced by electric current has attracted extensive attention as an efficient method of controlling the magnetization in nanomagnetic structures. SOT-induced magnetization reversal is usually achieved with the aid of an in-plane bias magnetic field. In this paper, we show that by selecting a film stack with weak out-of-plane magnetic anisotropy, field-free SOT-induced switching can be achieved in micron sized multilayers. Using direct current, deterministic bipolar magnetization reversal is obtained in Pt/[Co/Ni]2/Co/Ta structures. Kerr imaging reveals that the SOT-induced magnetization switching process is completed via the nucleation of reverse domain and propagation of domain wall in the system.
The spin-orbit torque (SOT) effective fields, namely field-like and damping-like terms, depend on the thicknesses of heavy metal (HM) and ferromagnetic metal (FM) layers, in a stack comprising of HM/FM/HM or oxide. In this work, we report on the dependence of the SOT effective fields on the magnetization uniformity in the wires comprising of Ta/Co/Pt layer structure. SOT dependence on magnetization uniformity dependence was investigated by concurrent variation of the magnetization uniformity in Co layer and characterization of the SOT effective fields in each wire which excludes the layer thickness dependence influences. Our experimental results reveal that the field-like term decreases while the damping-like term increases with increasing Co magnetization uniformity. The magnetization uniformity influence on the effective fields is attributed to the spin Hall effect, which contributes to the SOT.
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