Abstract. Recent thinning of glaciers over the Himalayas (sometimes referred to as the third polar region) have raised concern on future water supplies since these glaciers supply water to large river systems that support millions of people inhabiting the surrounding areas. Black carbon (BC) aerosols, released from incomplete combustion, have been increasingly implicated as causing large changes in the hydrology and radiative forcing over Asia and its deposition on snow is thought to increase snow melt. In India BC emissions from biofuel combustion is highly prevalent and compared to other regions, BC aerosol amounts are high. Here, we quantify the impact of BC aerosols on snow cover and precipitation from 1990 to 2010 over the Indian subcontinental region using two different BC emission inventories. New estimates indicate that Indian BC emissions from coal and biofuel are large and transport is expected to expand rapidly in coming years. We show that over the Himalayas, from 1990 to 2000, simulated snow/ice cover decreases by ∼0.9% due to aerosols. The contribution of the enhanced Indian BC to this decline is ∼36%, similar to that simulated for 2000 to 2010. Spatial patterns of modeled changes in snow cover and precipitation are similar to observations (from 1990 to 2000), and are mainly obtained with the newer BC estimates.

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Abstract. Recent thinning of glaciers over the Himalayas (sometimes referred to as the third polar region) have raised concern on future water supplies since these glaciers supply water to large river systems that support millions of people inhabiting the surrounding areas. Black carbon (BC) aerosols, released from incomplete combustion, have been increasingly implicated as causing large changes in the hydrology and radiative forcing over Asia and its deposition on snow is thought to increase snow melt. In India BC from biofuel combustion is highly prevalent and compared to other regions, BC aerosol amounts are high. Here, we quantify the impact of BC aerosols on snow cover and precipitation from 1990 to 2010 over the Indian subcontinental region using two different BC emission inventories. New estimates indicate that Indian BC from coal and biofuel are large and transport is expected to expand rapidly in coming years. We show that over the Himalayas, from 1990 to 2000, simulated snow/ice cover decreases by ~0.9% due to aerosols. The contribution of the enhanced Indian BC to this decline is ~30%, similar to that simulated for 2000 to 2010. Spatial patterns of modeled changes in snow cover and precipitation are similar to observations (from 1990 to 2000), and are mainly obtained with the newer BC estimates.

We present a zinc|ferricyanide hybrid flow battery that achieves extensive first-pass desalination while simultaneously supplying electrical energy (10 Wh/L). We demonstrate 85% salt removal from simulated seawater (35 g/L NaCl) and 86% from hypersaline brine (100 g/L NaCl), together with reversible battery operation over 100 h with high round-trip efficiency (84.8%). The system has a high operating voltage (E 0 = +1.25 V), low specific energy consumption (2.11 Wh/L for 85% salt removal), and a desalination flux (4.7 mol/m 2 •h) on par with that of reverse osmosis membranes. Salt removal was similarly effective at higher feed salinities, for which reverse osmosis becomes physically impossible because of the pressure required. The results have positive implications for regions that rely on desalination for their freshwater needs, especially where sea salinity is high. Alternatively, the battery may also be useful in minimal liquid discharge wastewater treatment if operated as a brine concentrator.

In this study, we characterize the impacts of COVID-19 on air pollution using NO2 and Aerosol Optical Depth (AOD) from TROPOMI and MODIS satellite datasets for 41 cities in India. Specifically, our results suggested a 13% NO2 reduction during the lockdown (March 25–May 3rd, 2020) compared to the pre-lockdown (January 1st–March 24th, 2020) period. Also, a 19% reduction in NO2 was observed during the 2020-lockdown as compared to the same period during 2019. The top cities where NO2 reduction occurred were New Delhi (61.74%), Delhi (60.37%), Bangalore (48.25%), Ahmedabad (46.20%), Nagpur (46.13%), Gandhinagar (45.64) and Mumbai (43.08%) with less reduction in coastal cities. The temporal analysis revealed a progressive decrease in NO2 for all seven cities during the 2020 lockdown period. Results also suggested spatial differences, i.e., as the distance from the city center increased, the NO2 levels decreased exponentially. In contrast, to the decreased NO2 observed for most of the cities, we observed an increase in NO2 for cities in Northeast India during the 2020 lockdown period and attribute it to vegetation fires. The NO2 temporal patterns matched the AOD signal; however, the correlations were poor. Overall, our results highlight COVID-19 impacts on NO2, and the results can inform pollution mitigation efforts across different cities of India.

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[1] A Geographical Information System (GIS) based methodology has been used to construct the black carbon (BC) emission inventory for the Indian geographical region. The distribution of emissions from a broader level to a spatial resolution of 1°Â 1°grid has been carried out by considering micro level details and activity data of fossil fuels and bio-fuels. Our calculated total BC emissions were 1343.78 Gg and 835.50 Gg for the base years 2001 and 1991 respectively with a decadal growth of around 61%, which is highly significant. The district level analysis shows a diverse spatial distribution with the top 10% emitting districts contributing nearly 50% of total BC emission. Coal contributes more than 50% of total BC emission. All the metropolitan cities show high BC emissions due to high population density giving rise to high vehicular emissions and more demand of energy.