We present the first experimental demonstration of quantum-enhanced detection at xray wavelengths. We show that x-ray pairs that are generated by spontaneous downconversion can be used for the generation of heralded x-ray photons and measure directly the sub-Poissonian statistics of the single photons by using photon number resolving detectors. We utilize the properties of the strong time-energy correlations of the down converted photons to demonstrate the ability to improve the visibility and the signal-to-noise ratio of an image with a small number of photons in an environment with a noise level that is higher than the signal by many orders of magnitude. In our work we demonstrate a new protocol for the measurement of quantum effects with x-rays using advantages such as background free measurements that the x-ray regime offers for experiments aiming at testing fundamental concepts in quantum optics. *Sharon.shwartz@biu.ac.il

Nonlinear interactions between X-rays and long wavelength radiation can be used as a powerful atomic-scale probe for light-matter interactions and for properties of valence electrons. However, reported X-ray nonlinear effects were small and their observations required tremendous efforts. Here we report the observation of strong nonlinearities in parametric down-conversion (PDC) of X-rays to long wavelength radiation in gallium arsenide and lithium niobate crystals, with efficiencies about 4 orders of magnitude stronger than the efficiencies measured in any material studied before. Furthermore, we show that the efficiency in the ferroelectric phase of strontium barium niobite is two orders of magnitude stronger than in its paraelectric phase. This observation suggests that the lack of inversion symmetry is the origin for the strong observed nonlinearity. Additionally, we demonstrate the ability to use the effect for the investigation of the spectral response of non-centrosymmetric materials at wavelengths ranging from infrared to soft X-rays.

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