More than 130 observation days of the horizontal and vertical extent of Saharan dust intrusions over Europe during the period May 2000 to December 2002 were studied by means of a coordinated lidar network in the frame of the European Aerosol Research Lidar Network (EARLINET). The number of dust events was greatest in late spring, summer, and early autumn periods, mainly in southern (S) and southeastern (SE) Europe. Multiple aerosol dust layers of variable thickness (300–7500 m) were observed. The center of mass of these layers was located in altitudes between 850 and 8000 m. However, the mean thickness of the dust layer typically stayed around 1500–3400 m and the corresponding mean center of mass ranged from 2500 to 6000 m. In exceptional cases, dust aerosols reached northwestern (NW), northern (N), or northeastern (NE) Europe, penetrating the geographical area located between 4°W–28°E (longitude) and 38°N–58°N (latitude). Mean aerosol optical depths (AOD), extinction-to-backscatter ratios (lidar ratios, LR), and linear depolarization ratios of desert aerosols ranged from 0.1 to 0.25 at the wavelength of 355 or 351 nm, 30 to 80 sr at 355 or 351 nm, and 10 to 25% at 532 nm, respectively, within the lofted dust plumes. In these plumes typical Saharan dust backscatter coefficients ranged from 0.5 to 2 Mm−1sr−1. Southern European stations presented higher variability of the LR values and the backscatter-related Ångström exponent values (BRAE) (LR: 20–100 sr; BRAE: −0.5 to 3) than northern ones (LR: 30–80 sr; BRAE: −0.5 to 1)

Abstract.A global vertically resolved aerosol data set covering more than 10 years of observations at more than 20 measurement sites distributed from 63 • N to 52 • S and 72 • W to 124 • E has been achieved within the Raman and polarization lidar network Polly NET . This network consists of portable, remote-controlled multiwavelength-polarization-Raman lidars (Polly) for automated and continuous 24/7 observations of clouds and aerosols. Polly NET is an independent, voluntary, and scientific network. All Polly lidars feature a standardized instrument design with different capabilities ranging from single wavelength to multiwavelength systems, and now apply unified calibration, quality control, and data analysis. The observations are processed in near-real time without manual intervention, and are presented online at polly.tropos.de. The paper gives an overview of the observations on four continents and two research vessels obtained with eight Polly systems. The specific aerosol types at these locations (mineral dust, smoke, dust-smoke and other dusty mixtures, urban haze, and volcanic ash) are identified by their Ångström exponent, lidar ratio, and depolarization ratio. The vertical aerosol distribution at the Polly NET locations is discussed on the basis of more than 55 000 automatically retrieved 30 min particle backscatter coefficient profiles at 532 nm as this operating wavelength is available for all Polly lidar systems. A seasonal analysis of measurements at selected sites revealed typical and extraordinary aerosol conditions as well as seasonal differences. These studies show the potential of Polly NET to support the establishment of a global aerosol climatology that covers the entire troposphere.

Abstract. We investigate the potential of polarization lidar to provide vertical profiles of aerosol parameters from which cloud condensation nucleus (CCN) and ice nucleating particle (INP) number concentrations can be estimated. We show that height profiles of particle number concentrations n 50,dry considering dry aerosol particles with radius > 50 nm (reservoir of CCN in the case of marine and continental non-desert aerosols), n 100,dry (particles with dry radius > 100 nm, reservoir of desert dust CCN), and of n 250,dry (particles with dry radius > 250 nm, reservoir of favorable INP), as well as profiles of the particle surface area concentration s dry (used in INP parameterizations) can be retrieved from lidar-derived aerosol extinction coefficients σ with relative uncertainties of a factor of 1.5-2 in the case of n 50,dry and n 100,dry and of about 25-50 % in the case of n 250,dry and s dry . Of key importance is the potential of polarization lidar to distinguish and separate the optical properties of desert aerosols from non-desert aerosol such as continental and marine particles. We investigate the relationship between σ , measured at ambient atmospheric conditions, and n 50,dry for marine and continental aerosols, n 100,dry for desert dust particles, and n 250,dry and s dry for three aerosol types (desert, non-desert continental, marine) and for the main lidar wavelengths of 355, 532, and 1064 nm. Our study is based on multiyear Aerosol Robotic Network (AERONET) photometer observations of aerosol optical thickness and column-integrated particle size distribution at Leipzig, Germany, and Limassol, Cyprus, which cover all realistic aerosol mixtures. We further include AERONET data from field campaigns in Morocco, Cabo Verde, and Barbados, which provide pure dust and pure marine aerosol scenarios. By means of a simple CCN parameterization (with n 50,dry or n 100,dry as input) and available INP parameterization schemes (with n 250,dry and s dry as input) we finally compute profiles of the CCN-relevant particle number concentration n CCN and the INP number concentration n INP . We apply the method to a lidar observation of a heavy dust outbreak crossing Cyprus and a case dominated by continental aerosol pollution.

[1] A strategy for European Aerosol Research Lidar Network (EARLINET) correlative measurements for Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) has been developed. These EARLINET correlative measurements started in June 2006 and are still in progress. Up to now, more than 4500 correlative files are available in the EARLINET database. Independent extinction and backscatter measurements carried out at high-performance EARLINET stations have been used for a quantitative comparison with CALIPSO level 1 data. Results demonstrate the good performance of CALIPSO and the absence of evident biases in the CALIPSO raw signals. The agreement is also good for the distribution of the differences for the attenuated backscatter at 532 nm ((CALIPSO-EARLINET)/EARLINET (%)), calculated in the 1-10 km altitude range, with a mean relative difference of 4.6%, a standard deviation of 50%, and a median value of 0.6%. A major Saharan dust outbreak lasting from 26 to 31 May 2008 has been used as a case study for showing first results in terms of comparison with CALIPSO level 2 data. A statistical analysis of dust properties, in terms of intensive optical properties (lidar ratios, Ångström exponents, and color ratios), has been performed for this observational period. We obtained typical lidar ratios of the dust event of 49 ± 10 sr and 56 ± 7 sr at 355 and 532 nm, respectively. The extinction-related and backscatter-related Ångström exponents were on the order of 0.15-0.17, which corresponds to respective color ratios of 0.91-0.95. This dust event has been used to show the methodology used for the investigation of spatial and temporal representativeness of measurements with polar-orbiting satellites.