Silicon carbide (SiC) supports surface phonons in the infrared region of the electromagnetic spectrum where these modes can be thermally emitted. Additionally, the magnitude, spectrum, and direction of thermal radiation from SiC can be controlled by engineering this material at the sub-wavelength scale. For these reasons, SiC nanopillars are of high interest for thermal-radiation tuning. So far, theoretical and experimental studies of thermal emission from SiC nanopillars have been limited to long-pitch arrays with a microscale interpillar spacing. It is not clear how far-field thermal emission from SiC nanopillars is affected when the interparticle spacing reduces to the nanometer scale, where the near-field interaction between adjacent nanopillars arises and the array becomes zero order. In this Letter, we study physical mechanisms of far-field thermal radiation from zero-order arrays of silicon-carbide nanopillars with a nanoscale interpillar spacing. We show that the increased volume of thermal emitters and thermal radiation of the hybrid waveguide-surface-phonon-polariton mode from zero-order arrays increase the spectral emissivity of silicon carbide to values as large as 1 for a wide range of angles. The enhanced, dispersion-less thermal emission from a zero-order SiC array of nano-frustums with an optimized interspacing of 300 nm is experimentally demonstrated. Our study provides insight into thermal radiation from dense nanostructures and has significant implications for thermal management of electronic devices and energy harvesting applications.
Thermal emission of localized surface phonons (LSPhs)
from nanostructures
of polaritonic materials is a promising mechanism for tuning the spectrum
of near-field thermal radiation. Previous studies have theoretically
shown that thermal emission of LSPhs results in narrow-band peaks
in the near-field spectra, whose spectral locations can be modulated
by changing the dimensions of the nanostructure. However, near-field
thermal emission of LSPhs has not been experimentally explored yet.
In this study, we measure the spectrum of near-field thermal radiation
from arrays of 6H-silicon carbide (6H-SiC) nanopillars using an internal-reflection-element
based spectroscopy technique. We present an experimental demonstration
of thermal emission of the transverse dipole, quadrupole, and octupole
as well as longitudinal monopole from 6H-SiC nanopillars at a near-field
distance from the array. We show that the spectral locations of the
longitudinal monopole and transverse dipole are significantly affected
by the near-field coupling between neighboring nanopillars as well
as the intercoupling of the nanopillars and the substrate. We also
experimentally demonstrate that the spectrum of near-field thermal
radiation from 6H-SiC nanopillar arrays can be tuned by varying the
dimensions of the nanopillars, providing an opportunity for designing
emitters with tailored near-field thermal radiation.
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