GERMANYStrong electronic correlations can produce remarkable phenomena such as metal-insulator transitions 1 and greatly enhance superconductivity 2 , thermoelectricity 3 , or optical non-linearity 4 . In correlated systems, spatially varying charge textures also amplify magnetoelectric effects 5 or electroresistance in mesostructures 6 . However, how spatially varying spin textures may influence electron transport in the presence of correlations remains unclear. Here we demonstrate a very large topological Hall effect (THE) 7,8 in thin films of a lightly electron-doped charge-transfer insulator, (Ca, Ce)MnO3. Magnetic force microscopy reveals the presence of magnetic bubbles, whose density vs. magnetic field peaks near the THE maximum, as is expected to occur in skyrmion systems 9 . The THE critically depends on carrier concentration and diverges at low doping, near the metal-insulator transition. We discuss the strong amplification of the THE by correlation effects and give perspectives for its non-volatile control by electric fields.* manuel.bibes@cnrs-thales.fr these authors contributed equally to the manuscript.
Using hybrid piezoelectric-magnetic systems we have generated large amplitude magnetization waves mediated by magnetoelasticity with up to 25 degrees variation in the magnetization orientation. We present direct imaging and quantification of both standing and propagating acoustomagnetic waves with different wavelengths, over large distances up to several millimeters in a nickel thin film.
Due to their large magneto-optic responses, rare-earth-doped yttrium iron garnets, Y 3 Fe 5 O 12 (YIG), are highly regarded for their potential in photonics and magnonics. Here, we consider the case of Ce-doped YIG (Ce-YIG) thin films, in which substitutional Ce 3+ ions are magnetic because of their 4f 1 ground state. In order to elucidate the impact of Ce substitution on the magnetization of YIG, we have carried out soft x-ray spectroscopy measurements on Ce-YIG films. In particular, we have used the element specificity of x-ray magnetic circular dichroism to extract the individual magnetization curves linked to Ce and Fe ions. Our results show that Ce doping triggers a selective charge transfer from Ce to the Fe tetrahedral sites in the YIG structure. This, in turn, causes a disruption of the electronic and magnetic properties of the parent compound, reducing the exchange coupling between the Ce and Fe magnetic moments and causing atypical magnetic behavior. Our work is relevant for understanding magnetism in rare-earth-doped YIG and, eventually, may enable a quantitative evaluation of the magneto-optical properties of rare-earth incorporation into YIG.
We have uncovered a giant gyrotropic magneto-optical response for doped ferromagnetic manganite La_{2/3}Ca_{1/3}MnO_{3} around the near room-temperature paramagnetic-to-ferromagnetic transition. At odds with current wisdom, where this response is usually assumed to be fundamentally fixed by the electronic band structure, we point to the presence of small polarons as the driving force for this unexpected phenomenon. We explain the observed properties by the intricate interplay of mobility, Jahn-Teller effect, and spin-orbit coupling of small polarons. As magnetic polarons are ubiquitously inherent to many strongly correlated systems, our results provide an original, general pathway towards the generation of magnetic-responsive gigantic gyrotropic responses that may open novel avenues for magnetoelectric coupling beyond the conventional modulation of magnetization.
Efforts have been recently made to use remanence plots in exchange-bias studies. However, since the two remnant magnetizations of a biased loop may differ, this technique cannot be applied in its classical form. This work extends it to systems with shifted loops and shows that the number of distinct plots is significantly increased. The approach was probed on Co/IrMn exchange bias films. Possible discrepancies between experiment and theory are pointed out and discussed. The adaptation of the model presented here enables it to become one of the few accessible techniques for rapid and accurate evaluation of magnetic interactions in biased systems. V C 2013 AIP Publishing LLC.
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