Over the past two years, the heat treatment of corundum involving lattice diffusion of beryllium (Be) at temperatures over 1800°C has become a major issue in the gem trade. Although initially only orange to orangy pink ("padparadscha"-like) sapphires were seen, it is now known that a full range of corundum colors, including yellow and blue as well as ruby, have been produced or altered by this treatment. An extension of the current understanding of the causes of color in corundum is presented to help explain the color modifications induced by Be diffusion. Empirical support is provided by Bediffusion experiments conducted on corundum from various geographic sources. Examination of hundreds of rough and faceted Be-diffused sapphires revealed that standard gemological testing will identify many of these treated corundums, although in some instances costly chemical analysis by mass spectrometry is required. Potential new methods are being investigated to provide additional identification aids, as major laboratories develop special nomenclature for describing this treatment.
Excited states in 38,40,42 Si nuclei have been studied via in-beam γ-ray spectroscopy with multinucleon removal reactions. Intense radioactive beams of 40 S and 44 S provided at the new facility of the RIKEN Radioactive Isotope Beam Factory enabled γ-γ coincidence measurements. A prominent γ line observed with an energy of 742 (8) 23.20.Lv, 27.40.+z, 29.38.Db Shell closures and collectivity are important properties that characterize the atomic nucleus. Interchange of their dominance along isotopic or isotonic chains has attracted much attention. The recent extension of the research frontier to nuclei far away from the valley of stability has revealed several new phenomena for neutronor proton-number dependent nuclear structure. For example, a weakening or even disappearance of shell closures occur in several neutron-rich nuclei at N = 8 [1][2][3] and N = 20 [4][5][6]. A well known example in the case of N = 20 is the so-called 'island of inversion ' [7] located around the neutron-rich nucleus 32 Mg. The low excitation energy of the first 2 + state E x (2 + 1 ) and large E2 transition probability [4][5][6] clearly indicate shell quenching in 32 Mg despite the fact that N = 20 is traditionally a magic number. The next magic number, N = 28, which appears due to the f 7/2 -f 5/2 spin-orbit splitting, has also been explored [8][9][10][11][12][13]. Weakening of the shell closure is seen by the decrease of the 2 With proton number Z = 14 and neutron number N = 28, the nuclear structure of 42 Si is of special interest. A simple but important question that arises is whether the weakening of the N = 28 shell closure continues, causing an enhancement of nuclear collectivity, or if shell stability is restored owing to a possible doubly magic structure. A study on 42 Si was made by a two-proton removal reaction experiment with radioactive 44 S beams at the NSCL [15]. The small two-proton removal cross sec-
Intermediate-energy Coulomb excitation measurements are performed on the N ! 40 neutron-rich nuclei 66;68 Fe and 64 Cr. The reduced transition matrix elements providing a direct measure of the quadrupole collectivity BðE2; 2 þ 1 ! 0 þ 1 Þ are determined for the first time in 68 Fe 42 and 64 Cr 40 and confirm a previous recoil distance method lifetime measurement in 66 Fe 40 . The results are compared to state-ofthe-art large-scale shell-model calculations within the full fpgd neutron orbital model space using the Lenzi-Nowacki-Poves-Sieja effective interaction and confirm the results of the calculations that show these nuclei are well deformed. DOI: 10.1103/PhysRevLett.110.242701 PACS numbers: 25.70.De, 27.50.+e For many decades the nuclear shell structure originally proposed by Mayer [1] and Jensen and coworkers [2], where energy gaps are predicted at specific nucleon numbers, was a paradigm of nuclear physics, as it was consistent with the experimental findings at or near the valley of beta stability. However, with the possibility of producing more exotic nuclei, the traditional magic numbers have been observed to be weakened or to disappear while new subshell gaps have emerged. In particular, the role of the proton-neutron tensor interaction has been recognized as driving changes in the shell structure [3]. Alterations to the effective single-particle orbital gaps can lead to enhanced particle-hole excitations, which are supported by deformation and pairing effects, and may give rise to new regions of well-developed nuclear deformation.A region of recent interest is that of the neutron-rich isotopes near N ¼ 40, below the 28 Ni isotopes. In many ways structurally similar to the ''island of inversion '' nuclei near N ¼ 20 [4], the Fe and Cr isotopes in this region have been experimentally observed to exhibit increasingly collective behavior, rather than the near-magic behavior naively expected assuming a robust N ¼ 40 subshell gap. In a schematic way, the development of collectivity moving from 28 Ni to 26 Fe and 24 Cr is understood as a result of a narrowing of the N ¼ 40 subshell closure and the enhancement of quadrupole collectivity through promotion of neutron pairs across the subshell gap. With the removal of protons from the 1f 7=2 orbital, the attractive tensor and central parts of the p-n interaction between 1f 7=2 proton holes and neutrons in the 1g 9=2 and 2d 5=2 orbits pull these neutron single-particle levels down in energy. At the same time, the repulsive tensor ð1f 7=2 Þ À1 À 1f 5=2 interaction dominates over the central attractive p-n interaction and drives the neutron 1f 5=2 orbital up, effectively quenching the N ¼ 40 gap. Looking at it another way, adding 12 neutrons to 48 Ca produces a gapless 60 Ca; as protons are added in the 1f 7=2 orbit, the repulsive interaction between the 1f 7=2 protons and the 1g 9=2 and 2d 5=2 neutrons and the strongly attractive 1f 7=2 -1f 5=2 interaction opens the N ¼ 40 gap up to its value in 68 Ni. The disappearance of the N ¼ 40 gap towards 60 Ca supports ...
The γ-ray strength function and level density in the quasi-continuum of 151,153 Sm have been measured using BGO shielded Ge clover detectors of the STARLiTeR system. The Compton shields allow for an extraction of the γ strength down to unprecedentedly low γ energies of ≈ 500 keV. For the first time an enhanced lowenergy γ-ray strength has been observed in the rare-earth region. In addition, for the first time both the upbend and the well known scissors resonance have been observed simultaneously for the same nucleus. HauserFeshbach calculations show that this strength enhancement at low γ energies could have an impact of 2-3 orders of magnitude on the (n,γ) reaction rates for the r-process nucleosynthesis.
Neutron-rich N=22, 24, 26 magnesium isotopes were studied via in-beam γ-ray spectroscopy at the RIKEN Radioactive Isotope Beam Factory following secondary fragmentation reactions on a carbon target at ≈200 MeV/nucleon. In the one- and two-proton removal channels from 39Al and 40Si beams, two distinct γ-ray transitions were observed in 38Mg, while in the one-proton removal reaction from 37Al a new transition was observed in addition to the known 2(1)(+)→0(g.s.)(+) decay. From the experimental systematics and comparison to theoretical predictions it is concluded that the transitions belong to the 2(1)(+)→0(g.s.)(+) and 4(1)(+)→2(1)(+) decays in 36Mg and 38Mg, respectively. For 34Mg, previously reported 2(1)(+) and 4(1)(+) level energies were remeasured. The deduced E(4(1)(+))/E(2(1)(+)) ratios for 34,36,38Mg of 3.14(5), 3.07(5), and 3.07(5) are almost identical and suggest the emergence of a large area of deformation extending from the N=20 to the N=28 shell quenching.
Obtaining reliable data for nuclear reactions on unstable isotopes remains an extremely important task and a formidable challenge. Neutron capture cross sections-crucial ingredients for models of astrophysical processes, national security applications, and simulations of nuclear energy generation-are particularly elusive, as both projectile and target in the reaction are unstable. We demonstrate a new method for determining cross sections for neutron capture on unstable isotopes, using ^{87}Y(n,γ) as a prototype. To validate the method, a benchmark experiment is carried out to obtain the known ^{90}Zr(n,γ) cross section analogously. Our approach, which employs an indirect ("surrogate") measurement combined with theory, can be generalized to a larger class of nuclear reactions. It can be used both with traditional stable-beam experiments and in inverse kinematics at rare-isotope facilities.
The neutron-capture reaction plays a critical role in the synthesis of the elements in stars and is important for societal applications including nuclear power generation and stockpile-stewardship science. However, it is difficult -if not impossible -to directly measure neutron capture cross sections for the exotic, short-lived nuclei that participate in these processes. In this Letter we demonstrate a new technique which can be used to indirectly determine neutron-capture cross sections for exotic systems. This technique makes use of the (d, p) transfer reaction, which has long been used as a tool to study the structure of nuclei. Recent advances in reaction theory, together with data collected using this reaction, enable the determination of neutron-capture cross sections for short-lived nuclei. A benchmark study of the 95 Mo(d, p) reaction is presented, which illustrates the approach and provides guidance for future applications of the method with short-lived isotopes produced at rare isotope accelerators.Essentially all of the heavy elements are synthesized in astrophysical environments by processes that involve neutron capture. The slow neutron-capture process (the s process) occurs predominantly in the low neutron flux in AGB stars, yielding a nucleosynthesis path that typically deviates only one or two neutrons from β-stability. In contrast, the rapid neutron-capture process (the r process) involves exotic neutron-rich nuclei and requires explosive stellar scenarios with high neutron fluences. The r process is responsible for the creation of roughly half of the elements between iron and bismuth and synthesizes heavy nuclei through the rapid production of neutronrich nuclei via neutron capture and subsequent β decay.The recent observation of the gravitational waves associated with a neutron-star merger [1], and the subsequent kilonova understood to be powered by the decay of lanthanides [2,3], demonstrated that neutron-star mergers are an important r -process site, especially for the heaviest elements. However, r -process abundance patterns are sensitive to astrophysical conditions (cf. [4]). In a "cold" r process (which could occur in a neutron star merger or with the highly accelerated neutrino-driven winds following a core-collapse supernova), equilibrium between neutron capture (n, γ) and photo-dissociation (γ, n) rapidly breaks down, so the rate at which neutron capture proceeds will affect the final r -process abun-dance pattern. The timescales of the cold r process are such that competition between neutron capture and β decay occurs during the bulk of the r -process nucleosynthesis. Neutron-capture rates on unstable nuclei affect the final observed abundance patterns even in the traditional "hot" r process (thought to occur in the neutrinodriven winds in a proto-neutron star resulting from a core-collapse supernova) during the eventual freeze-out, when (n, γ) (γ, n) equilibrium no longer occurs. Accordingly, neutron capture is influential in determining the final r -process abundance pattern, especia...
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