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Shallow, maritime cumuli are ubiquitous over much of the tropical oceans, and characterizing their properties is important to understanding weather and climate. The Rain in Cumulus over the Ocean (RICO) field campaign, which took place during November 2004–January 2005 in the trades over the western Atlantic, emphasized measurements of processes related to the formation of rain in shallow cumuli, and how rain subsequently modifies the structure and ensemble statistics of trade wind clouds. Eight weeks of nearly continuous S-band polarimetric radar sampling, 57 flights from three heavily instrumented research aircraft, and a suite of ground- and ship-based instrumentation provided data on trade wind clouds with unprecedented resolution. Observational strategies employed during RICO capitalized on the advances in remote sensing and other instrumentation to provide insight into processes that span a range of scales and that lie at the heart of questions relating to the cause and effects of rain from shallow maritime cumuli.

SUMMARYParticle size distributions measured by the UK C-130 aircraft in ice stratiform cloud around the British Isles are analysed. Probability distribution functions over large scales show that the zeroth, second and fourth moments (equivalent to concentration, ice water content and radar reflectivity) as well as mean particle size have monomodal distributions. Rescaling of the size distributions requiring knowledge of two moments reveals a 'universal' distribution that has been fitted with analytically integrable functions. The existence of the 'universal' distribution implies that two-moment microphysics schemes are adequate to represent particle size distributions (PSDs). In large-scale models it may be difficult to predict two moments, and so power laws between moments have been found as functions of in-cloud temperature. This means that a model capable of predicting ice water content and temperature can predict ice PSDs to use for calculations requiring knowledge of the size distribution (e.g. precipitation rate, radar reflectivity) or to make direct use of the power laws relating moments of the size distribution.

Ice particle interarrival times have been measured with a fast forward scattering spectrometer probe (FSSP). The distribution of interarrival times is bimodal instead of the exponential distribution expected for a Poisson process. The interarrival time modes are located at ϳ10 Ϫ2 and ϳ10 Ϫ4 s. This equates to horizontal spacings on both the centimeter and meter scales. The characteristics of the interarrival times are well modeled by a Markov chain process that couples together two independent Poisson processes operating at different scales. The possibility that ice crystals shattering on the probe tip causes the bimodal interarrival times is explored and cannot be ruled out. If the observations are indicating real spacings of particles in clouds, then the observations show very localized (centimeter scale) concentrations of ϳ100 s cm Ϫ3 embedded within an average concentration of typically ϳ1 cm Ϫ3. If the localized high concentrations are produced by the ice crystals shattering, then the concentration measured by the FSSP is overcounted by a factor of 5 in the worst case measured here, but more typically by a factor of 2. This uncertainty in concentration will adversely affect the predicted radiative influence of these clouds.

Abstract. The VAMOS Ocean-Cloud-Atmosphere-Land Regional Experiment (VOCALS-REx) was conducted from 15 October to 15 November 2008 in the South East Pacific (SEP) region to investigate interactions between land, sea and atmosphere in this unique tropical eastern ocean environment and to improve the skill of global and regional models in representing the region. This study synthesises selected aircraft, ship and surface site observations from VOCALSREx to statistically summarise and characterise the atmospheric composition and variability of the Marine Boundary Layer (MBL) and Free Troposphere (FT) along the 20 • S parallel between 70 • W and 85 • W. Significant zonal gradients in mean MBL sub-micron aerosol particle size and composition, carbon monoxide, sulphur dioxide and ozone were seen over the campaign, with a generally more variable and polluted coastal environment and a less variable, more pristine remote maritime regime. Gradients in aerosol and trace gas concentrations were observed to be associated with strong gradients in cloud droplet number. The FT wasCorrespondence to: G. Allen (grant.allen@manchester.ac.uk) often more polluted in terms of trace gases than the MBL in the mean; however increased variability in the FT composition suggests an episodic nature to elevated concentrations. This is consistent with a complex vertical interleaving of airmasses with diverse sources and hence pollutant concentrations as seen by generalised back trajectory analysis, which suggests contributions from both local and longrange sources. Furthermore, back trajectory analysis demonstrates that the observed zonal gradients both in the boundary layer and the free troposphere are characteristic of marked changes in airmass history with distance offshore -coastal boundary layer airmasses having been in recent contact with the local land surface and remote maritime airmasses having resided over ocean for in excess of ten days. Boundary layer composition to the east of 75 • W was observed to be dominated by coastal emissions from sources to the west of the Andes, with evidence for diurnal pumping of the Andean boundary layer above the height of the marine capping inversion. Analysis of intra-campaign variability in atmospheric composition was not found to be significantly correlated with observed low-frequency variability in the large scale flow pattern; campaign-average interquartile ranges of Published by Copernicus Publications on behalf of the European Geosciences Union. 5238 G. Allen et al.: South East Pacific composition during VOCALS-REx CO, SO 2 and O 3 concentrations at all longitudes were observed to dominate over much smaller differences in median concentrations calculated between periods of different flow regimes. The campaign climatology presented here aims to provide a valuable dataset to inform model simulation and future process studies, particularly in the context of aerosolcloud interaction and further evaluation of dynamical processes in the SEP region for conditions analogous to those during VOCALS-REx....