Abstract. Dielectric barrier discharges (BDs) are known to operate in two distinctive modes. Filamentary mode of DB is characterized by large number of short lasting spatially bounded microdischarges. This type of discharge is typical for most cases of BDs at atmospheric pressure. Under some specific conditions another form of BD may arise. In this mode plasma covers uniformly the whole electrode area. This mode is usually referred to as diffuse or homogeneous mode of BD.This work presents studies of filamentary mode of BD in argon and its transition to the diffuse mode by ammonia addition. The discharges were investigated by the means of Cross Correlation Spectroscopy (CCS). Particularly the influence of electrode shape, discharge gap and influence of ammonia admixture on discharge development were studied. The measurement offers results with high temporal and spatial resolution which are useful for comparison with results of numerical models.The obtained results include the electrical current measurement of discharge in several ammonia admixtures to argon. The diffuse discharge appeared at ammonia admixture above 3 vol% The observed propagation of streamer in discharge in pure argon for two different electrode configuration is presented. When compared to discharge in pure argon the streamer velocity is decreased for 0.1 vol% ammonia admixture. With increasing ammonia concentration the streamer velocity increases again. The behaviour of presented impurities was observed and the results are included in this report. The basic model of the discharge kinetic is included. For reduced electric field below 10 Td the electron drift is much higher in argon ammonia mixture than in pure argon.
The spectral and spatial characteristics of three-dimensional radiation transfer across an arc column of 0.08 m long, typical in high-voltage gas blast circuit breakers, has been studied in detail. The arc column under study corresponds to an instantaneous current of 15 kA in SF6 gas at a pressure of 10 bar. Our results show that to calculate the radiative flux divergence (as a volumetric energy source), only a segment of the arc column of 0.024 m in thickness needs to be considered to attain an accuracy of better than 90%. Photons with a frequency lower than 21015 Hz (150 nm in wavelength) can travel a considerable distance (> 0.02 m) with an intensity attenuation factor of 0.2-0.8. Above 21015 Hz, only photons from the continuum spectrum can travel up to 0.015 m and line emission is absorbed within a distance of typically 0.0005 m, i.e. the arcing gas is optically thick to these photons. The gas within a cross-section of the arc column can be divided into a net emission core and a net absorption zone. 55% - 75% of the radiation emitted from the core is reabsorbed. The starting position of the net absorption zone sits within the temperature interval of 75% to 80% of the maximum temperature on the axis. The quantitative information from this work is expected to serve as baseline data for developing improved approximate models for radiation transfer calculation in SF6 switching arcs.
In radiation modeling of thermal plasmas non-grey models are applied where the radiative transport is described in several frequency bands (spectral intervals). Hereby mean absorption coefficients have to be calculated by a spectral integration procedure, providing a constant mean absorption coefficient for each band. Depending on the number of bands, one or more integration boundaries have to be selected in order to do the integration. In this paper we evaluate the influence of the selection of these integration boundaries on the mean absorption coefficient and the also radiation transfer by applying the mean absorption coefficients in a radiation transport model. Using a simplified twoband model we demonstrate that the selection of the integration boundary has a large impact on the total model accuracy. We show that in some cases selecting a band boundary right at the frequency where the continuum absorption shows a jump can introduce a significant error into the radiation calculation. The process of the integration interval selection thus demands a global optimization procedure to properly evaluate the boundaries of each frequency band.
Atmospheric pressure dielectric barrier discharge (DBD) in Ar/H2 gas feed with C2H2 or CH4 admixture was studied at room and high temperature of 680 °C by plasma diagnostics (electrical measurements, fast camera imaging, and optical emission spectroscopy). It was shown that filamentary DBD in pure Ar or Ar/H2 can be converted into homogeneous discharge by an acetylene admixture. Fast intensified charge-coupled device (ICCD) camera proved that this homogeneous discharge is an atmospheric pressure glow discharge (APGD) at room temperature whereas at high temperature the discharge mode switches at every half-period between APGD and atmospheric pressure Townsend discharge. The high temperature discharges (610–710 °C) in Ar/H2/C2H2 and Ar/H2/CH4 were also investigated with respect to a surface bound deposition of carbon nanotubes using 5 nm thick iron layer as a catalyst. CNTs were deposited without any dedicated catalyst pretreatment phase. The quality of CNTs, namely, their density, vertical alignment, and width of the diameter distribution, was better for the C2H2 gas feed and higher temperatures.
The objective of this work is to compare the accuracy of several approximate models of radiative properties for the prediction of radiative transfer in air arc plasma at the temperatures in the range of 300 - 25 000 K and the pressure of 0.1 MPa. Calculated absorption coefficients are used to generate the parameters of different models. The radiative transfer inside the cylindrically symmetrical air plasma with prescribed temperature profile was studied. The equation of radiative transfer was solved using the P1 and SP3 approximations, calculated radiative source term in the energy equation (net emission) was compared with results obtained by spectral integration.
Recently the technologies based on atmospheric pressure plasma sources become very promising tool for the control of surface properties of solids while the desirable bulk properties are kept. In this work the surface barrier discharge operated at atmospheric pressure was used for deposition of thin protective hydrophobic films from mixture of nitrogen with C 4 F 8 on the paper substrate. The plasma parameters were investigated by means of optical emission spectroscopy. Surface properties of the deposited thin films were studied by means of the contact angle measurements. The colorimetric parameters such as whiteness, yellowness or brightness of samples were measured in its deposited state and also in UV exposed states.PACS : 52.77.Dq
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