This paper presents a combined 2D numerical and experimental study of the influence of N 2 admixture on the dynamics of a He-N 2 discharge in the 10 cm long dielectric tube of a plasma gun set-up. First, the comparison between experiments and simulations is carried out on the ionization front propagation velocity in the tube. The importance of taking into account a detailed kinetic scheme for the He-N 2 mixture in the simulations to obtain a good agreement with the experiments is put forward. For the μs driven plasma gun, the two-and three-body Penning reactions occurring in the plasma column behind the ionization front, are shown to play a key role on the discharge dynamics. In the experiments and simulations, the significant influence of the amplitude of the applied voltage on the ionization front propagation velocity is observed. As the amount of N 2 varies, simulation results show that the ionization front velocity, depends on a complex coupling between the kinetics of the discharge, the photoionization and the 2D structure of the discharge in the tube. Finally, the time evolution of axial and radial components of the electric field measured by an electro-optic probe set outside the tube are compared with simulation results. A good agreement is obtained on both components of the electric field. In the tube, simulations show that the magnitude of the axial electric field on the discharge axis depends weakly on the amount of N 2 conversely to the magnitude of the off-axis peak electric field. Both, simulations and first measurements in the tube or within the plasma plume show peak electric fields of the order of 45 kV•cm −1 .

This work investigates the dynamical charging of a surface under exposure of a non-equilibrium plasma jet at atmospheric pressure through a quantitative comparison between modeling and experiments. We show using mono-polar pulses with variable pulse duration and amplitude that the charging time (i.e. the time from impact of the ionization wave till the fall of the high voltage pulse) is a crucial element determining the plasma-surface interaction. This is done through direct measurements of the electric field induced inside the target using the optical diagnostic technique called Mueller polarimetry and comparison with the electric field calculated using a 2D fluid model of the plasma jet interaction with the target in the same conditions as in the experiments. When the charging time is kept relatively short (less than 100 ns), the surface spreading of the discharge and consequent surface charge deposition are limited. When it is relatively long (up to microseconds), the increased surface spreading and charge deposition significantly change the electric field to which the target is exposed during the charging time and when the applied voltage returns to zero.

This work addresses plasma chemistry in the core of a vortex-stabilized microwave discharge for CO2 conversion numerically, focusing on the pressure-dependent contraction dynamics of this plasma. A zero-dimensional model is presented for experimental conditions in a pressure range between 60 and 300 mbar and a temperature range between 3000 and 6500 K. Monte Carlo flux (MCF) simulations, which describe electron kinetics, are self-consistently coupled to the plasma chemistry model. The simulation results show that an increase in pressure is accompanied by a transition in neutral composition in the plasma core: from a significant amount of CO2 and O2 at low pressures to a O/CO/C mixture at high pressures, the composition being determined mostly by thermal equilibrium and by transport processes. The change of temperature and composition with pressure lead to higher ionisation coefficient and more atomic ion composition in the plasma core. These changes result in an increase in ionisation degree in the plasma core from 10−5 to 10−4. These factors are shown to be fundamental to drive contraction in the CO2 microwave discharge.

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The interaction of kHz μs-pulsed atmospheric pressure He jets with metallic targets is studied through simulations and experiments, focusing on the differences between floating and grounded targets. It is shown that the electric potential of the floating target is close to grounded in the instants after the impact of the discharge, but rises to a high voltage, potentially more than half of the applied voltage, at the end of the 1 μs pulse. As a result, a return stroke takes place after the discharge impact with both grounded and floating targets, as a redistribution between the high voltage electrode and the low voltage target. Electric field, electron temperature and electron density in the plasma plume are higher during the pulse with grounded target than with floating target, as gradients of electric potential progressively dissipate in the latter case. Finally, at the fall of the pulse, another electrical redistribution takes place, with higher intensity with the highly-charged floating target than with the grounded target. It is shown that this phenomenon can lead to an increase in electric field, electron temperature and electron density in the plume with floating target.

This work presents a study of the influence of dielectric permittivity on the interaction between a positive pulsed He plasma jet and a 0.5 mm-thick dielectric target, using a validated two-dimensional numerical model. Six different targets are studied: five targets at floating potential with relative permittivities r = 1, 4, 20, 56 and 80; and one grounded target of permittivity r = 56. The temporal evolution of the charging of the target and of the electric field inside the target are described, during the pulse of applied voltage and after its fall. It is found that the order of magnitude of the electric field inside the dielectric targets is the same for all floating targets with r ≥ 4. For all these targets, during the pulse of applied voltage, the electric field perpendicular to the target and averaged through the target thickness, at the point of discharge impact, is between 1 and 5 kV cm −1. For the two remaining targets (r = 1 and grounded target with r = 56), the field is significantly higher than for all the other floating targets.

This paper presents 2D simulations of atmospheric pressure discharges in helium with N 2 and O 2 admixtures, propagating in a dielectric tube between a point electrode and a grounded metallic target. For both positive and negative polarities, the propagation of the first ionization front is shown to correspond to a peak of the absolute value of the axial electric field inside the tube, but also outside the tube. After the impact on the metallic target, a rebound front is shown to propagate from the target to the point electrode. This rebound front is 2-3 times faster than the first ionization front. Close to the high voltage point, this rebound front corresponds to a second peak of the absolute value of the axial electric field. Close to the target, as the first ionization and rebound fronts are close in time, only one peak is observed. The dynamics of the absolute value of the radial component of electric field outside the tube is shown to present an increase during the first ionization front propagation and a fast decrease corresponding to the propagation of the rebound front. These time evolutions of the electric field components are in agreement with experiments. Finally, we have shown that the density of metastable He * in 99% He-1% N 2 and 99% He-1% O 2 atmospheric pressure discharges are very close. Close to the grounded target, the peak density of reactive species is significantly increased due to the synergy between the first ionization and rebound fronts, as observed in experiments. Similar results are obtained for both voltage polarities, but the peak density of metastable He * close to the target is shown to be two times less in negative polarity than in positive polarity.

Plasma jets are sources of repetitive and stable ionization waves, meant for applications where they interact with surfaces of different characteristics. As such, plasma jets provide an ideal testbed for the study of transient reproducible streamer discharge dynamics, particularly in inhomogeneous gaseous mixtures, and of plasma-surface interactions. This topical review addresses the physics of plasma jets and their interactions with surfaces through a pedagogical approach. The state-of-the-art of numerical models and diagnostic techniques to describe helium jets is presented, along with the benchmarking of different experimental measurements in literature and recent efforts for direct comparisons between simulations and measurements. This exposure is focused on the most fundamental physical quantities determining discharge dynamics, such as the electric field, the mean electron energy and the electron number density, as well as the charging of targets. The physics of plasma jets is described for jet systems of increasing complexity, showing the effect of the different components (tube, electrodes, gas mixing in the plume, target) of the jet system on discharge dynamics. Focusing on coaxial helium kHz plasma jets powered by rectangular pulses of applied voltage, physical phenomena imposed by different targets on the discharge, such as discharge acceleration, surface spreading, the return stroke and the charge relaxation event, are explained and reviewed. Finally, open questions and perspectives for the physics of plasma jets and interactions with surfaces are outlined.