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57 Fe Mössbauer effect spectra were collected at 4.2 K for the Ho(Fe 1−x Co x ) 2 C15 Laves phases. The hyperfine interaction parameters, i.e. isomer shift, the magnetic hyperfine field and the quadrupole interaction parameter, were determined for the individual Fe/Co nearest neighbourhoods of iron atoms and also as average values for the sample as bulk. As a result of Fe/Co substitution, Slater-Pauling-type dependences for magnetic hyperfine fields corresponding to both the local area and the sample as bulk were observed, and a linear correlation between the local magnetic hyperfine field and the average magnetic hyperfine field was observed. Magnetic moments of atoms were obtained from band structure calculations using the full-potential linearized augmented plane wave method. The magnetic hyperfine field obtained from the experiment correlates linearly (but separately for weak and strong ferromagnetic areas) with the magnetic moment calculated per transition metal atom.

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