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Molecular design of magnetically active graphene nanoscale structures is an emerging field of research. The key goal of this research is to produce graphene nanoribbons and graphene quantum dots with specified electronic, optical and magnetic properties. The review considers methods for the synthesis of spin-labelled polycyclic aromatic hydrocarbons, which are homologous precursors of graphene nanostructures, and discusses the advances and prospects of the design of magnetically active graphene materials. The bibliography includes 134 references.

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