Soft ionic conductors, such as hydrogels and ionogels, have enabled stretchable and transparent ionotronics, but they suffer from key limitations inherent to the liquid components, which may leak and evaporate. Here, novel liquid‐free ionic conductive elastomers (ICE) that are copolymer networks hosting lithium cations and associated anions via lithium bonds and hydrogen bonds are demonstrated, such that they are intrinsically immune from leakage and evaporation. The ICEs show extraordinary mechanical versatility including excellent stretchability, high strength and toughness, self‐healing, quick self‐recovery, and 3D‐printability. More intriguingly, the ICEs can defeat the conflict of strength versus toughness—a compromise well recognized in mechanics and material science—and simultaneously overcome the conflict between ionic conductivity and mechanical properties, which is common for ionogels. Several liquid‐free ionotronics based on the ICE are further developed, including resistive force sensors, multifunctional ionic skins, and triboelectric nanogenerators (TENGs), which are not subject to limitations of previous gel‐based devices, such as leakage, evaporation, and weak hydrogel–elastomer interfaces. Also, the 3D printability of the ICEs is demonstrated by printing a series of structures with fine features. The findings offer promise for a variety of ionotronics requiring environmental stability and durability.
Inspired by natural creatures, soft robots possess the unique advantages of large actuation and excellent adaptability. Untethered designs of soft robots are drawing more attention to researchers, but current research is limited. Also, there is an increasing need to improve the performance of bio-mimetic robots. This work describes an untethered soft robotic jellyfish with high mobility that can mimic a natural jellyfish’s performance. The electrode of the robotic jellyfish is made by sandwiching carbon grease between two layers of dielectric elastomer film. The frame of the material, where six plastic paddles are attached, is made from a silicone elastomer. The robotic jellyfish has a maximum recorded swim speed of up to 1 cm s−1, with a peak thrust force of 0.000 12 N. A finite element simulation is developed to study the performance of the robotic jellyfish in a theoretical manner. By embedding a compact remote-controlled power source, the robotic jellyfish is made autonomous. In this case, the max peak speed is around 0.5 cm s−1. Ultimately, the working principles of the bio-mimetic robotic jellyfish can be useful in field studies and to guide the design of soft robots and flexible devices.
Soft robots driven by stimuli-responsive materials have their own unique advantages over traditional rigid robots such as large actuation, light weight, good flexibility and biocompatibility. However, the large actuation of soft robots inherently co-exists with difficulty in control with high precision. This article presents a soft artificial muscle driven robot mimicking cuttlefish with a fully integrated on-board system including power supply and wireless communication system. Without any motors, the movements of the cuttlefish robot are solely actuated by dielectric elastomer which exhibits muscle-like properties including large deformation and high energy density. Reinforcement learning is used to optimize the control strategy of the cuttlefish robot instead of manual adjustment. From scratch, the swimming speed of the robot is enhanced by 91% with reinforcement learning, reaching to 21 mm/s (0.38 body length per second). The design principle behind the structure and the control of the robot can be potentially useful in guiding device designs for demanding applications such as flexible devices and soft robots.
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