We report the implementation and operation of novel superhigh-reflectivity negative-dispersion dielectric mirrors for use in tunable ultrafast laser systems. The mirror structure is divided into two distinct regions: an underlying superhigh-reflectivity dielectric quarter-wavelength stack and an overlying negative-dispersion section consisting of only a few layers and forming simple multiple Gires-Tournois interferometers. The example that we present was designed for operation from 800 to 900 nm and has a near-constant group-delay dispersion of -40 fs(2) and a peak reflectivity greater than 99.99%. We show a comparison of the predicted and the measured mirror performance and application of these mirrors in a mode-locked Ti:sapphire laser tunable from 805 to 915 nm.
A 100-kHz mode-locked Ti:sapphire-seeded regenerative amplifier pumping an optical parametric amplifier generates femtosecond pulses tunable from 470 to 710 nm. This output was compressed with a pair of prisms to bandwidth-limited pulses of 80- to 40-fs duration and more than 150 nJ of energy. These tunable pulses were then bandwidth expanded through self-phase modulation in bulk material and further compressed to less than 30-fs duration.
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