As artificial intelligence calls for novel energy-efficient hardware, neuromorphic computing systems based on analog resistive switching memory (RSM) devices have drawn great attention recently. Different from the well-studied binary RSMs, the analog RSMs are featured by a continuous and controllable conductance-tuning ability and thus are capable of combining analog computing and data storage at the device level. Although significant research achievements on analog RSMs have been accomplished, there have been few works demonstrating large-scale neuromorphic systems. A major bottleneck lies in the reliability issues of the analog RSM, such as endurance and retention degradation and read/write noises and disturbances. Owing to the complexity of resistive switching mechanisms, studies on the origins of reliability degradation and the corresponding optimization methodology face many challenges. In this article, aiming on the high-performance neuromorphic computing applications, we provide a comprehensive review on the status of reliability studies of analog RSMs, the reliability requirements, and evaluation criteria and outlook for future reliability research directions in this field.

Leakage interference between memory cells is the primary obstacle for enlarging X‐point memory arrays. Metal‐filament threshold switches, possessing excellent selectivity and low leakage current, are developed in series with memory cells to reduce sneak path current and lower power consumption. However, these selectors typically have limited on‐state currents (≤10 µA), which are insufficient for memory RESET operations. Here, a strategy is proposed to achieve sufficiently large RESET current (≈2.3 mA) by introducing highly ordered Ag nanodots to the threshold switch. Compared to the Ag thin film case, Ag nanodots as active electrode could avoid excessive Ag atoms migration into solid electrolyte during operations, which causes stable conductive filament growth. Furthermore, Ag nanodots with rapid thermal processing contribute to forming multiple weak Ag filaments at a lower voltage and then spontaneous rupture as the applied voltage reduced, according to quantized conductance and simulation analysis. Impressively, the Ag nanodots based threshold switch, which is bidirectional and truly electroforming‐free, demonstrates extremely high selectivity >10 9 , ultralow leakage current <1 pA, very steep slope of 0.65 mV dec −1 , and good thermal stability up to 200 °C, and further represents significant suppression of leakage currents and excellent performances for SET/RESET operations in the one‐selector‐one‐resistor configuration.

No abstract