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Abstract. Emission inventories are the quantification of pollutants from different sources. They provide important information not only for climate and weather studies but also for urban planning and environmental health protection. We developed an open-source model (called Vehicular Emissions Inventory – VEIN v0.2.2) that provides high-resolution vehicular emissions inventories for different fields of studies. We focused on vehicular sources at street and hourly levels due to the current lack of information about these sources, mainly in developing countries.The type of emissions covered by VEIN are exhaust (hot and cold) and evaporative considering the deterioration of the factors. VEIN also performs speciation and incorporates functions to generate and spatially allocate emissions databases. It allows users to load their own emission factors, but it also provides emission factors from the road transport model (Copert), the United States Environmental Protection Agency (EPA) and Brazilian databases. The VEIN model reads, distributes by age of use and extrapolates hourly traffic data, and it estimates emissions hourly and spatially. Based on our knowledge, VEIN is the first bottom–up vehicle emissions software that allows input to the WRF-Chem model. Therefore, the VEIN model provides an important, easy and fast way of elaborating or analyzing vehicular emissions inventories under different scenarios. The VEIN results can be used as an input for atmospheric models, health studies, air quality standardizations and decision making.

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Worldwide, urbanization constitutes a major and growing driver of global change and a distinctive feature of the Anthropocene. Thus, urban development paths present opportunities for technological and societal transformations towards energy efficiency and decarbonization, with benefits for both greenhouse gas (GHG) and air pollution mitigation. This requires a better understanding of the intertwined dynamics of urban energy and land use, emissions, demographics, governance, and societal and biophysical processes. In this study, we address several characteristics of urbanization in Santiago (33.5°S, 70.5°W, 500 m a.s.l.), the capital city of Chile. Specifically, we focus on the multiple links between mobility and air quality, describe the evolution of these two aspects over the past 30 years, and review the role scientific knowledge has played in policy-making. We show evidence of how technological measures (e.g., fuel quality, three-way catalytic converters, diesel particle filters) have been successful in decreasing coarse mode aerosol (PM10) concentrations in Santiago despite increasing urbanization (e.g., population, motorization, urban sprawl). However, we also show that such measures will likely be insufficient if behavioral changes do not achieve an increase in the use of public transportation. Our investigation seeks to inform urban development in the Anthropocene, and our results may be useful for other developing countries, particularly in Latin America and the Caribbean where more than 80% of the population is urban.

The changing composition of the atmosphere, driven by anthropogenic emissions, is the cause of anthropogenic climate change as well as deteriorating air quality. Emission inventories are essential to understand the contribution of various human activities, model and predict the changing atmospheric composition, and design cost-effective mitigation measures. At present, national emission inventories in South America (SA) focus on Greenhouse Gases (GHG) as part of their obligations to the United Nations Framework Convention for Climate Change (UNFCC) within the framework of their national communications. Emission inventories other than for GHG in SA focus mainly on growing urban areas and megacities. Therefore, studies examining air quality at national, regional or continental scales in SA depend on (down-scaled) global emission inventories. This paper examines the emission estimates of air pollutants from various global inventories for five SA countries, namely Argentina, Brazil, Chile, Colombia and Peru. A more detailed analysis is conducted for the EDGAR and ECLIPSE emission inventories, in particular against local city-scale inventories of a major city in each country. Although total emissions between down-scaled global inventories and local city inventories are often comparable, large discrepancies exist between the sectoral contributions. This is critical as the mitigation of poor air quality will depend on addressing the right sources. Potential sources of discrepancies between global and local inventories include the spatial distribution proxies, difference in emission factors used and/or the use of generic statistical country data when estimating emissions. This highlights the importance of using local information when generating national emission inventories, especially for air quality modeling and development of effective mitigation measures. This work represents a first step towards an increased understanding of the strength and weaknesses of emissions information in SA.

Rapid vehicle growth in developing nations makes it necessary for these nations to address the transportation and environmental impacts of on-road mobile sources. To estimate the air quality impact of their fleets, many nations have adopted modified versions of U.S. or European emissions models or factors. In most cases, these models can lead to significant errors in emissions estimates. To address this problem, a new on-road mobile source emissions model, called the international vehicle emissions (IVE) model, designed for use in developing countries has been developed. The IVE model was developed jointly by researchers at the International Sustainable Systems Research Center and the University of California at Riverside. The IVE model uses local vehicle technology distributions, power-based driving factors, vehicle soak distributions, and meteorological factors to tailor the model to the local situation. In addition, an intensive 2-week field study was designed to collect the necessary fleet and activity data to populate the model with critical local information. The IVE model, along with the field study process, has proved highly effective in providing an improved estimate of mobile source emissions in an urban area and allows the effective analysis of local policy options. The studies have served to transfer tools and knowledge on the process of creating and improving mobile source inventories in an efficient manner. The rationale behind the development of the model, the development and application of the field studies, an overview of the results obtained to date, and planned next steps are described in this paper.

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