High mobility, solution-processed field-effect transistors are important building blocks for flexible electronics. Here we demonstrate the alignment of semiconducting, colloidal ZnO nanorods by a simple solvent evaporation technique and achieve high electron mobilities in field-effect transistors at low operating voltages by electrolyte-gating with ionic liquids. The degree of alignment varies with nanorod length, concentration and solvent evaporation rate. We find a strong dependence of electron mobility on the degree of alignment but less on the length of the nanorods. Maximum field-effect mobilities reach up to 9 cm(2) V(-1) s(-1) for optimal alignment. Because of the low process temperature (150 °C), ZnO nanorod thin films are suitable for application on flexible polymer substrates.
In this article we discuss the synthesis of four new low band-gap co-polymers based on the diketopyrrolopyrrole (DPP) and benzotriazole (BTZ) monomer unit.
We consider a quench in a free-fermion chain by joining two homogeneous half-chains via a defect. The time evolution of the entanglement negativity is studied between adjacent segments surrounding the defect. In case of equal initial fillings, the negativity grows logarithmically in time and essentially equals one-half of the Rényi mutual information with index α = 1/2 in the limit of large segments. In sharp contrast, in the biased case one finds a linear increase followed by the saturation at an extensive value for both quantities, which is due to the backscattering from the defect and can be reproduced in a quasiparticle picture. Furthermore, a closer inspection of the subleading corrections reveals that the negativity and the mutual information have a small but finite difference in the steady state. Finally, we also study a similar quench in the XXZ spin chain via density-matrix renormalization group methods and compare the results for the negativity to the fermionic case.
We investigate the dynamics of the XXZ spin chain after a geometric quench, which is realized by connecting two half-chains prepared in their ground states with zero and maximum magnetizations, respectively. The profiles of magnetization after the subsequent time evolution are studied numerically by density-matrix renormalization group methods, and a comparison to the predictions of generalized hydrodynamics yields a very good agreement. We also calculate the profiles of entanglement entropy and propose an ansatz for the noninteracting XX case, based on arguments from conformal field theory. In the general interacting case, the propagation of the entropy front is studied numerically both before and after the reflection from the chain boundaries. Finally, our results for the magnetization fluctuations indicate a leading order proportionality relation to the entanglement entropy.
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