We report the complete GNO solar neutrino results for the measuring periods GNO III, GNO II, and GNO I. The result for GNO III (last 15 solar runs) is View the MathML source[54.3−9.3+9.9(stat)±2.3(syst)]SNU(1σ)(1σ) or View the MathML source[54.3−9.6+10.2(incl. syst)] SNU (1σ ) with errors combined. The GNO experiment is now terminated after altogether 58 solar exposure runs that were performed between 20 May 1998 and 9 April 2003. The combined result for GNO (I + II + III) is View the MathML source[62.9−5.3+5.5(stat)±2.5(syst)] SNU (1σ ) or View the MathML source[62.9−5.9+6.0] SNU (1σ ) with errors combined in quadrature. Overall, gallium based solar observations at LNGS (first in GALLEX, later in GNO) lasted from 14 May 1991 through 9 April 2003. The joint result from 123 runs in GNO and GALLEX is [69.3±5.5(incl. syst)] SNU[69.3±5.5(incl. syst)] SNU (1σ). The distribution of the individual run results is consistent with the hypothesis of a neutrino flux that is constant in time. Implications from the data in particle- and astrophysics are reiterated
Age is a key parameter when deducing the history of plutonium material, i.e. the plutonium produced in the nuclear reactors. This is of vital importance, when a smuggled plutonium sample has been seized and the origin has to be determined. A methodology is described which allows accurately to determine the age of plutonium material by thermal ionisation mass spectrometry using independent parent/daughter relations. This has been demonstrated for Reference Materials of known ages as well as for real samples. The already established method using gamma spectrometry is compared to this.
Lead and strontium isotope ratios were used for the origin assessment of uranium ore concentrates (yellow cakes) for nuclear forensic purposes. A simple and low-background sample preparation method was developed for the simultaneous separation of the analytes followed by the measurement of the isotope ratios by multicollector inductively coupled plasma mass spectrometry (MC-ICPMS). The lead isotopic composition of the ore concentrates suggests applicability for the verification of the source of the nuclear material and by the use of the radiogenic (207)Pb/(206)Pb ratio the age of the raw ore material can be calculated. However, during data interpretation, the relatively high variation of the lead isotopic composition within the mine site and the generally high contribution of natural lead as technological contamination have to be carefully taken into account. The (87)Sr/(86)Sr isotope ratio is less prone to the variation within one mine site and less affected by the production process, thus it was found to be a more purposeful indicator for the origin assessment and source verification than the lead. The lead and strontium isotope ratios measured and the methodology developed provide information on the initial raw uranium ore used, and thus they can be used for source attribution of the uranium ore concentrates.
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