Plasmonic systems based on metal nanoparticles on a metal film with high optical absorption have generated great interests for surface‐enhanced Raman scattering (SERS). In this study, we prepare a broadband‐visible light absorber consisting Au nanotriangles on the surface of a continuous optically opaque gold film separated with a dielectric SiO2 layer, which is a typical metal‐insulator‐metal (MIM) system, and demonstrate it as an efficient SERS substrate. The MIM nanostructure, prepared using nanosphere lithography with a very large area, shows a broadband with absorption exceeding 90% in the wavelength regime of 630–920 nm. We observe an average SERS enhancement factor (EF) as large as 4.9 × 106 with a 22‐fold increase compared to a single layer of Au nanotriangles directly on a quartz substrate. A maximum SERS EF can be achieved by optimizing the thicknesses of the dielectric layer to control the optical absorption. Owing to the simple, productive, and inexpensive fabrication technique, our MIM nanostructure could be a potential candidate for SERS applications. Copyright © 2015 John Wiley & Sons, Ltd.
Transversal magneto-optical Kerr effect (TMOKE) has potential practical applications, such as biosensors, magnetic imaging, and date storage. However, these potential applications have been restricted by its very weak response (about 0.1%) in natural ferromagnetic metal material such as Fe, Co and Ni. Fortunately, with the development of the nanofabrication techniques, surface plasmons (SPs) are one of the effective strategies to solve this problem due to their special ability to manipulate light on a nanoscale and concentrate the electromagnetic energy near the metal/dielectric interface. Herein, in order to enhance the TMOKE response, we propose that a periodic gold strips array is embedded into a magnetic dielectric film of bismuth iron garnet (BIG), which is supported by a quartz substrate. Using the finite element method, we numerically study the optical properties of our proposed microstructure and the corresponding evolution of the TMOKE responses due to the coupled optical modes dependent on the structural parameters. Particularly, by optimizing the embedded depth of metal grating, a dramatic enhancement of TMOKE response (about 3.6%) is achieved when the embedded depth reaches up to 80 nm, accompanied with a high transmissivity about 22.6%, which is actually three time larger than that in the case that the gold strips are just patterned on the surface of the BIG film. As the embedding depth increases further, the TMOKE response will be weak. The relationship between the TMOKE response and the coupling efficiency of LSP resonance of the gold stripes and the waveguide (WG) mode supported by the BIG film are also discussed systematically. As the embedding depth increases up to 80 nm gradually, the coupling of the WG mode in BIG film with the LSP mode of the individual gold stripe becomes much stronger and forms a highly efficient Fano resonance, which leads to the fact that most of the electromagnetic field is localized in the BIG film and strong interaction with the BIG magnetic dielectric film, and thus, an enhancement of TMOKE response can be observed. However, when the embedded depth increases further, the uniformity of BIG film will be broken. In this case, WG mode cannot be supported by BIG film very well any more at the wavelength corresponding to excitation of the LSP, which results in a weakly coupling efficiency between LSP and WG mode. In this case, the Fano resonance cannot be formed and rare electromagnetic field can be localized in the BIG film, leading to a very weak light-magnetic dielectric film interaction and the weak TMOKE response. Our study proposes a new method to realize the amplification of weak TMOKE response by utilizing the plasmonic microstructure, which might have a potential application to designing the high-efficiency magneto-optical devices.
Herein, we propose a high-quality (Q) factor hybrid plasmonic nanocavity based on distributed Bragg reflectors (DBRs) with low propagation loss and extremely strong mode confinement. This hybrid plasmonic nanocavity is composed of a high-index cylindrical nanowire separated from a metal surface possessing shallow DBRs gratings by a sufficiently thin low-index dielectric layer. The hybrid plasmonic nanocavity possesses advantages such as a high Purcell factor (F p) of up to nearly 20000 and a gain threshold approaching 266 cm−1 at 1550 nm, promising a greater potential in deep sub-wavelength lasing applications.
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