Quantum phase is not a direct observable and is usually determined by
interferometric methods. We present a method to map complete electron wave
functions, including internal quantum phase information, from measured
single-state probability densities. We harness the mathematical discovery of
drum-like manifolds bearing different shapes but identical resonances, and
construct quantum isospectral nanostructures possessing matching electronic
structure but divergent physical structure. Quantum measurement (scanning
tunneling microscopy) of these "quantum drums" [degenerate two-dimensional
electron states on the Cu(111) surface confined by individually positioned CO
molecules] reveals that isospectrality provides an extra topological degree of
freedom enabling robust quantum state transplantation and phase extraction.Comment: Published 8 February 2008 in Science; 13 page manuscript (including 4
figures) + 13 page supplement (including 6 figures); supplementary movies
available at http://mota.stanford.ed
We have performed a detailed investigation of the photoluminescence pressure dependence of heteroepitaxial GaN thin films on sapphire substrates. A comparison between as grown GaN on sapphire and free-standing GaN membranes, created using a laser assisted substrate liftoff process, revealed that the presence of the sapphire substrate leads to an energy gap pressure coefficient reduction of approximately 5%. This result agrees with the numerical simulations presented in this article. We established that the linear pressure coefficient of free-standing GaN is 41.4±0.2 meV/GPa, and that the deformation potential of the energy gap is −9.36±0.04 eV. Our results also suggest a new, lower value of the pressure derivative for the bulk modulus of GaN (B′=3.5).
The energies of photo-and electroluminescence transitions in In x Ga 1Ϫx N quantum wells exhibit a characteristic ''blueshift'' with increasing pumping power. This effect has been attributed either to band-tail filling, or to screening of piezoelectric fields. We have studied the pressure and temperature behavior of radiative recombination in In x Ga 1Ϫx N/GaN quantum wells with xϭ0.06, 0.10, and 0.15. We find that, although the recombination has primarily a band-to-band character, the excitation-power induced blueshift can be attributed uniquely to piezoelectric screening. Calculations of the piezoelectric field in pseudomorphic In x Ga 1Ϫx N layers agree very well with the observed Stokes redshift of the photoluminescence. The observed pressure coefficients of the photoluminescence ͑25-37 meV/GPa͒ are surprisingly low, and, so far, their magnitude can only be partially explained.
The ability of the scanning tunnelling microscope to manipulate single atoms and molecules has allowed a single bit of information to be represented by a single atom or molecule. Although such information densities remain far beyond the reach of real-world devices, it has been assumed that the finite spacing between atoms in condensed-matter systems sets a rigid upper limit on information density. Here, we show that it is possible to exceed this limit with a holographic method that is based on electron wavefunctions rather than free-space optical waves. Scanning tunnelling microscopy and holograms comprised of individually manipulated molecules are used to create and detect electronically projected objects with features as small as approximately 0.3 nm, and to achieve information densities in excess of 20 bits nm-2. Our electronic quantum encoding scheme involves placing tens of bits of information into a single fermionic state.
A correlation of the local indium concentration measured on an atomic scale with luminescence properties of In x Ga 1-x N quantum wells reveals two different types of recombination mechanisms. A piezoelectric-field based mechanism is shown to dominate in samples with thick wells (L > 3 nm) of low indium concentration (x < 0.15-0.20). Spatial indium concentration fluctuations dominate luminescence properties in samples of higher indium concentrations in thinner wells. Quantum confinement is shown to have a major effect on the radiative recombination energy. A model is presented that relates the experimentally measured nano scale structural and chemical properties of quantum wells to the characteristics of the luminescence.
Atomic manipulation techniques have provided a bottom-up approach to investigating the unconventional properties and complex phases of strongly correlated electron materials. By engineering artificial systems containing tens to thousands of atoms with tailored electronic or magnetic properties, it has become possible to explore how quantum many-body effects emerge as the size of a system is increased from the nanoscale to the mesoscale. Here we investigate both theoretically and experimentally the quantum engineering of nanoscale Kondo lattices – Kondo droplets – exemplifying nanoscopic replicas of heavy-fermion materials. We demonstrate that by changing a droplet’s real-space geometry, we can not only create coherently coupled Kondo droplets whose properties asymptotically approach those of a quantum-coherent Kondo lattice, but also markedly increase or decrease the droplet’s Kondo temperature. Furthermore we report on the discovery of a new quantum phenomenon – the Kondo echo – a signature of droplets containing Kondo holes functioning as direct probes of spatially extended, quantum-coherent Kondo cloud correlations.
Alta Devices has successfully completed all milestones and deliverables established as part of the NREL PV incubator program. During the 18 months of this program, Alta has proven all key processes required to commercialize its solar module product. The incubator focus was on back end process steps directed at conversion of Alta's high quality solar film into high efficiency 1sun PV modules. This report will describe all program deliverables and the work behind each accomplishment.
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