Carbon nanoparticles (CNPs) have been considered as essential components for various applications including sensors, quantum dots, electrocatalysts, energy storages, lubrication, and functional coatings. Uniform and functional CNP materials can be obtained from candle soot. However, the production of CNPs from candle soot is not a continuous process, limiting the practical production and applications of such materials. Here, a rotatingdeposition and separation system for high-efficiency production of low-cost and high-quality CNPs from candle soot is presented. The characteristic of CNPs can be controlled by adjusting the system parameters. Moreover, obtained CNPs can act as photothermal superhydrophobic anti-icing coatings on various substrates. With a sliding angle of less than 3°, water drops can keep rolling off without further nucleation of ice. The reported preparing method is suitable for large-scale applications and various kinds of surfaces and shows great potentials in the growing demands of anti-icing.

A concise, protecting-group-free total synthesis of (-)-jiadifenolide, a synthetically challenging seco-prezizaane sesquiterpene with potent neurotrophic activity, is reported. The convergent route features a SmI2/H2O-mediated stereoselective reductive cyclization, an unprecedented formal [4 + 1] annulative tetrahydrofuran-forming reaction and programmed redox manipulations. The newly developed annulation of β-hydroxy aldehydes or ketones with lithium trimethylsilyldiazomethane provides access to a diverse array of multisubstituted tetrahydrofurans. The synthetic jiadifenolide exhibited weak cytotoxicity against five human cancer cell lines.

Thin film transistors (TFTs) with amorphous silicon films crystallized via continuous-wave green laser at a wavelength of 532 nm exhibit very different electrical characteristics in various crystallization regions, corresponding to the Gaussian energy density distribution of the laser beam. In the center region subjected to the highest energy density, the full melting scheme led to the best crystallinity of the polycrystalline silicon film, resulting in the highest field-effect mobility of 500 cm2 V−1 s−1. In contrast, the edge region that resulted in solid phase crystallization exhibited the worst mobility of 48 cm2 V−1 s−1 for the polycrystalline silicon TFTs.

All-solid-state batteries (ASSBs) are one of the most promising candidates for next-generation energy storage. In particular, ASSBs with sulfide solid-state electrolytes (SEs) offer high conductivity, rivaling those of liquid electrolytes...

The oxygen-plasma-functionalized carbon nanotube thin films on the flexible substrates as the pH sensing membranes of extended-gate field-effect transistors are proposed for the first time. The carbon nanotubes are ultrasonically sprayed onto the polyimide substrates followed by an oxygen-plasma functionalization. Such oxygen-plasma-treated carbon nanotube thin films (CNTFs) exhibit superior pH sensing characteristics with the sensitivity of 55.7 mV/pH and voltage linearity of 0.9996 in a wide sensing range of pH 1-13. Moreover, the excellent flexibility of carbon nanotube is also demonstrated and the oxygen-plasma-treated CNTFs still maintain the sensitivity of 53.6 mV/pH and voltage linearity of 0.9943 even after five-cycle bending test. These results reveal that the oxygen-plasma-treated CNTFs have great potentials in the practically disposal and wearable biosensor applications.Index Terms-Biosensors, carbon nanotube (CNT), extendedgate field-effect transistors (EGFETs), flexible substrates.