Intergrain tunneling magnetoresistance ͑TMR͒ subsisting up to room temperature has been observed for polycrystalline ceramics of Sr 2 FeReO 6 , which has ordered double perovskite structure with Curie temperature above 400 K. The first-principles band calculation predicts that Sr 2 FeReO 6 shows the half metallic ground state with the ferrimagnetic coupling of Fe and Re spins. The experimental results of electronic and magnetic properties are in accord with this picture. In fact, the magnitude of intergrain TMR with the magnetic field of 7 T at 4.2 and 300 K is as large as 21 and 7%, respectively, reflecting high spin polarization of carriers.
Epitaxial thin films of Sr2FeMoO6, that are ordered double perovskite with half-metallic nature, have been successfully prepared on SrTiO3 (001) and (111) substrates by pulsed laser deposition in a narrow window of the temperature and oxygen pressure. From the surface morphology analysis for the atomic scale step-and-terrace structures, the film growth is concluded to take place with the chemical formula as the growth unit when the ordering direction is normal to the surface. The films showed metallic conduction with ferromagnetic transition temperature above 400 K and intergrain tunneling type magnetoresistance even at room temperature.
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