After the severe accident in the Fukushima 1 nuclear power plant, a large amount of contaminated stagnant water has been produced in turbine buildings and surrounding areas. This rapid communication reports the calculation of the radionuclide inventory in the core, the collection of the measured inventory in the stagnant water, and the estimation of the radionuclide release ratios from the core to the stagnant water. The present evaluation is based on data obtained before June 3, 2011. It was revealed that the release ratios of tritium, iodine and cesium were several tens of percent, while those of strontium and barium were smaller by one or two orders of magnitude. These release ratios of the Fukushima accident were equivalent to those of the TMI 2 accident.

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Uranium, thorium, lead, and the lanthanides were automatically and sequentially separated with a single anion-exchange column. This separation was achieved using eluents consisting of a simple and highly pure acid mixture of HCl, HNO3, acetic acid, and HF. The elements of interest were separated from the major constituents, which included alkaline metal elements, alkaline earth metal elements, and iron. This simple and automatic system is driven with pressurized nitrogen gas and controlled using a computer program. An optimized separation was accomplished under the following conditions: a 50 mm long and 2 mm diameter column, 11 μm diameter anion-exchange resin, and a 35 μL min(-1) flow rate. Using this system, 50 ng of varied elements in a 100 μL feed solution were perfectly separated within 5 h with >400 decontamination factors and >95% yield. In order to evaluate the performance of this system, a reference powdered rock sample was separated using this system. Abundances of objective elements, including 0.23 ng of lutetium, were accurately determined without corrections of chemical recovery yield or subtraction of the process blank. This separation technique saves time and effort for chemical processing, and is useful for ultra-trace quantitative and isotopic analyses of elements in small environmental samples.

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