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Abstract. The observed cooling of the lower stratosphere over the last two decades has been attributed, in previous studies, largely to a combination of stratospheric ozone loss and carbon dioxide increase, and as such it is meant to provide one of the best pieces of evidence for an anthropogenic cause to climate change. This study shows how increases in stratospheric water vapour, inferred from available observations, may be capable of causing as much of the observed cooling as ozone loss does; as the reasons for the stratospheric water vapour increase are neither fully understood nor well characterized, it shows that it remains uncertain whether the cooling of the lower stratosphere can yet be fully attributable to human influences. In addition, the changes in stratospheric water vapour may have contributed, since 1980, a radiative forcing which enhances that due to carbon dioxide alone by 40%.

Abstract. To estimate the impact of emissions by road, aircraft and ship traffic on ozone and OH in the present-day atmosphere six different atmospheric chemistry models have been used. Based on newly developed global emission inventories for road, ship and aircraft emission data sets each model performed sensitivity simulations reducing the emissions of each transport sector by 5%. The model results indicate that on global annual average lower tropospheric ozone responds most sensitive to ship emissions (50.6%±10.9% of the total traffic induced perturbation), followed by road (36.7%±9.3%) and aircraft exhausts (12.7%±2.9%), respectively. In the northern upper troposphere between 200–300 hPa at 30–60° N the maximum impact from road and ship are 93% and 73% of the maximum effect of aircraft, respectively. The latter is 0.185 ppbv for ozone (for the 5% case) or 3.69 ppbv when scaling to 100%. On the global average the impact of road even dominates in the UTLS-region. The sensitivity of ozone formation per NOx molecule emitted is highest for aircraft exhausts. The local maximum effect of the summed traffic emissions on the ozone column predicted by the models is 0.2 DU and occurs over the northern subtropical Atlantic extending to central Europe. Below 800 hPa both ozone and OH respond most sensitively to ship emissions in the marine lower troposphere over the Atlantic. Based on the 5% perturbation the effect on ozone can exceed 0.6% close to the marine surface (global zonal mean) which is 80% of the total traffic induced ozone perturbation. In the southern hemisphere ship emissions contribute relatively strongly to the total ozone perturbation by 60%–80% throughout the year. Methane lifetime changes against OH are affected strongest by ship emissions up to 0.21 (± 0.05)%, followed by road (0.08 (±0.01)%) and air traffic (0.05 (± 0.02)%). Based on the full scale ozone and methane perturbations positive radiative forcings were calculated for road emissions (7.3±6.2 mWm−2) and for aviation (2.9±2.3 mWm−2). Ship induced methane lifetime changes dominate over the ozone forcing and therefore lead to a net negative forcing (−25.5±13.2 mWm−2).

As the global temperature increases with changing climate, precipitation rates and patterns are affected through a wide range of physical mechanisms. The globally averaged intensity of extreme precipitation also changes more rapidly than the globally averaged precipitation rate. While some aspects of the regional variation in precipitation predicted by climate models appear robust, there is still a large degree of intermodel differences unaccounted for. Individual drivers of climate change initially alter the energy budget of the atmosphere, leading to distinct rapid adjustments involving changes in precipitation. Differences in how these rapid adjustment processes manifest themselves within models are likely to explain a large fraction of the present model spread and better quantifications are needed to improve precipitation predictions. Here, the authors introduce the Precipitation Driver and Response Model Intercomparison Project (PDRMIP), where a set of idealized experiments designed to understand the role of different climate forcing mechanisms were performed by a large set of climate models. PDRMIP focuses on understanding how precipitation changes relating to rapid adjustments and slower responses to climate forcings are represented across models. Initial results show that rapid adjustments account for large regional differences in hydrological sensitivity across multiple drivers. The PDRMIP results are expected to dramatically improve understanding of the causes of the present diversity in future climate projections.

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Abstract. Changes in atmospheric ozone have occurred since the preindustrial era as a result of increasing anthropogenic emissions. Within ACCENT, a European Network of Excellence, ozone changes between 1850 and 2000 are assessed for the troposphere and the lower stratosphere (up to 30 km) by a variety of seven chemistry-climate models and three chemical transport models. The modeled ozone changes are taken as input for detailed calculations of radiative forcing.When only changes in chemistry are considered (constant climate) the modeled global-mean tropospheric ozone column increase since preindustrial times ranges from 7.9 DU to 13.8 DU among the ten participating models, while the stratospheric column reduction lies between 14.1 DU and 28.6 DU in the models considering stratospheric chemistry. The resulting radiative forcing is strongly dependent on the location and altitude of the modeled ozone change and varies between 0.25 Wm −2 and 0.45 Wm −2 due to ozone change in the troposphere and −0.123 Wm −2 and +0.066 Wm −2 due to the stratospheric ozone change.Correspondence to: M. Gauss (michael.gauss@geo.uio.no) Changes in ozone and other greenhouse gases since preindustrial times have altered climate. Six out of the ten participating models have performed an additional calculation taking into account both chemical and climate change. In most models the isolated effect of climate change is an enhancement of the tropospheric ozone column increase, while the stratospheric reduction becomes slightly less severe. In the three climate-chemistry models with detailed tropospheric and stratospheric chemistry the inclusion of climate change increases the resulting radiative forcing due to tropospheric ozone change by up to 0.10 Wm −2 , while the radiative forcing due to stratospheric ozone change is reduced by up to 0.034 Wm −2 .Considering tropospheric and stratospheric change combined, the total ozone column change is negative while the resulting net radiative forcing is positive.

We describe the historical evolution of the conceptualization, formulation, quantification, application, and utilization of “radiative forcing” (RF) of Earth’s climate. Basic theories of shortwave and longwave radiation were developed through the nineteenth and twentieth centuries and established the analytical framework for defining and quantifying the perturbations to Earth’s radiative energy balance by natural and anthropogenic influences. The insight that Earth’s climate could be radiatively forced by changes in carbon dioxide, first introduced in the nineteenth century, gained empirical support with sustained observations of the atmospheric concentrations of the gas beginning in 1957. Advances in laboratory and field measurements, theory, instrumentation, computational technology, data, and analysis of well-mixed greenhouse gases and the global climate system through the twentieth century enabled the development and formalism of RF; this allowed RF to be related to changes in global-mean surface temperature with the aid of increasingly sophisticated models. This in turn led to RF becoming firmly established as a principal concept in climate science by 1990. The linkage with surface temperature has proven to be the most important application of the RF concept, enabling a simple metric to evaluate the relative climate impacts of different agents. The late 1970s and 1980s saw accelerated developments in quantification, including the first assessment of the effect of the forcing due to the doubling of carbon dioxide on climate (the “Charney” report). The concept was subsequently extended to a wide variety of agents beyond well-mixed greenhouse gases (WMGHGs; carbon dioxide, methane, nitrous oxide, and halocarbons) to short-lived species such as ozone. The WMO and IPCC international assessments began the important sequence of periodic evaluations and quantifications of the forcings by natural (solar irradiance changes and stratospheric aerosols resulting from volcanic eruptions) and a growing set of anthropogenic agents (WMGHGs, ozone, aerosols, land surface changes, contrails). From the 1990s to the present, knowledge and scientific confidence in the radiative agents acting on the climate system have proliferated. The conceptual basis of RF has also evolved as both our understanding of the way radiative forcing drives climate change and the diversity of the forcing mechanisms have grown. This has led to the current situation where “effective radiative forcing” (ERF) is regarded as the preferred practical definition of radiative forcing in order to better capture the link between forcing and global-mean surface temperature change. The use of ERF, however, comes with its own attendant issues, including challenges in its diagnosis from climate models, its applications to small forcings, and blurring of the distinction between rapid climate adjustments (fast responses) and climate feedbacks; this will necessitate further elaboration of its utility in the future. Global climate model simulations of radiative perturbations by various agents have established how the forcings affect other climate variables besides temperature (e.g., precipitation). The forcing–response linkage as simulated by models, including the diversity in the spatial distribution of forcings by the different agents, has provided a practical demonstration of the effectiveness of agents in perturbing the radiative energy balance and causing climate changes. The significant advances over the past half century have established, with very high confidence, that the global-mean ERF due to human activity since preindustrial times is positive (the 2013 IPCC assessment gives a best estimate of 2.3 W m−2, with a range from 1.1 to 3.3 W m−2; 90% confidence interval). Further, except in the immediate aftermath of climatically significant volcanic eruptions, the net anthropogenic forcing dominates over natural radiative forcing mechanisms. Nevertheless, the substantial remaining uncertainty in the net anthropogenic ERF leads to large uncertainties in estimates of climate sensitivity from observations and in predicting future climate impacts. The uncertainty in the ERF arises principally from the incorporation of the rapid climate adjustments in the formulation, the well-recognized difficulties in characterizing the preindustrial state of the atmosphere, and the incomplete knowledge of the interactions of aerosols with clouds. This uncertainty impairs the quantitative evaluation of climate adaptation and mitigation pathways in the future. A grand challenge in Earth system science lies in continuing to sustain the relatively simple essence of the radiative forcing concept in a form similar to that originally devised, and at the same time improving the quantification of the forcing. This, in turn, demands an accurate, yet increasingly complex and comprehensive, accounting of the relevant processes in the climate system.

The response of climate to ozone perturbations caused by regional emissions of NOx or CO has been studied through a sequence of model simulations. Changes in O3 and OH concentrations due to emission perturbations in Europe and southeast Asia have been calculated with two global 3‐D chemical tracer models(CTMs; LMDzINCA and Oslo‐CTM2). The radiative transfer codes of three general circulation models (GCMs; ECHAM4, UREAD and LMD) have been used to calculate the radiative forcing of the O3 perturbations, and for a subset of the cases full GCM simulations have been performed with ECHAM4 and UREAD. The results have been aggregated to a global number in two ways: first, through integrating the global‐mean radiative forcing of a sustained step change in emissions, and second through a modified concept (SGWP*) which includes possible differences in the climate sensitivity of O3, CH4 and CO2 changes. In terms of change in global tropospheric O3 burden the two CTMs differ by less than 30%. Both CTMs show a higher north/south gradient in the sensitivity to changes in NOx emission than for CO. We are not able to conclude whether real O3 perturbations in general have a different climate sensitivity from CO2. However, in both GCMs high‐latitude emission perturbations lead to climate perturbations with higher (10–30%) climate sensitivities. The calculated SGWP*, for a 100 yr time horizon, are negative for three of the four CTM/GCM combinations for European emissions (−9.6 to +6.9), while for the Asian emissions the SGWP* (H= 100) is always positive (+2.9 to +25) indicating a warming. For CO the SGWP* values (3.8 and 4.4 for European and Asian emissions respectively, with only the Oslo‐CTM2/ECHAM4 model combination) are less regionally dependent. Our results support the view that for NOx, regionally different weighting factors for the emissions are necessary. For CO the results are more robust and one global number may be acceptable.