The β-decay properties of the neutron-deficient nuclei 25 Si and 26 P have been investigated at the GANIL/LISE3 facility by means of charged-particle and γ-ray spectroscopy. The decay schemes obtained and the Gamow-Teller strength distributions are compared to shell-model calculations based on the USD interaction. B(GT ) values derived from the absolute measurement of the β-decay branching ratios give rise to a quenching factor of the Gamow-Teller strength of 0.6. A precise half-life of 43.7 (6) ms was determined for 26 P , the β −(2)p decay mode of which is described.PACS. 29.30.Ep Charged-particle spectroscopy -29.30.Kv X-and gamma-ray spectroscopy -23.90.+w
The laser ion source project at the IGISOL facility, Jyväskylä, has motivated the development and construction of an rf sextupole ion beam guide (SPIG) to replace the original skimmer electrode. The SPIG has been tested both off-line and on-line in protoninduced fission, light-ion and heavy-ion induced fusion-evaporation reactions and, in each case, has been directly compared to the skimmer system. For both fission and light-ion induced fusion, the SPIG has improved the mass-separated ion yields by a factor of typically 4 to 8. Correspondingly, the transmission efficiency of both systems has been studied in simulations with and without space charge effects. The transport capacity of the SPIG has been experimentally determined to be ∼10 12 ions s −1 before space charge effects start to take effect. A direct comparison with the simulation has been made using data obtained via light-ion fusion evaporation. Both experiment and simulation show an encouraging agreement as a function of current extracted from the ion guide.
The feeding probability of 102;104;105;106;107 Tc, 105 Mo, and 101 Nb nuclei, which are important contributors to the decay heat in nuclear reactors, has been measured using the total absorption technique. We have coupled for the first time a total absorption spectrometer to a Penning trap in order to obtain sources of very high isobaric purity. Our results solve a significant part of a long-standing discrepancy in the component of the decay heat for 239 Pu in the 4-3000 s range. DOI: 10.1103/PhysRevLett.105.202501 PACS numbers: 23.40.Às, 27.60.+j, 28.41.Fr, 29.30.Kv Nuclear reactors provide a significant fraction of the world's electricity. A burgeoning population and an associated growth in economic activity suggest that world demand will double by 2050. Until now, the bulk of this has come from the burning of fossil fuels. There is general concern that reserves of fossil fuels are limited and their burning damages the environment. In particular, it contributes to the emission of large amounts of CO 2 . In this context, nuclear power, based on the fission process, will be less damaging to the environment. Accordingly there is now a renaissance in the building of nuclear power stations around the world. Modern reactor designs, based on many years of operating experience, are much more efficient, more economical, and safer than earlier designs. Although the basic principles are well established, we still lack certain information, such as a knowledge of the decay properties of specific nuclei that are important contributors to the heating of the reactor during and after operation. The estimation and control of the heat emitted by the decay of fission products plays a key role in the safe operation of reactors. The primary aim of this work is to study the decay properties of specific nuclei that are important contributors to this source of heat.Approximately 8% of the total energy generated during the fission process is related to the energy released in the natural decay of fission products, and is commonly called decay heat [1]. Once the reactor is shut down, the energy released in radioactive decay provides the main source of heating. Hence, coolant needs to be maintained after termination of the neutron-induced fission process in a reactor, and the form and extent of this essential requirement needs to be specified on the basis of decay-heat summation calculations. Decay heat varies as a function of time after shutdown and can be determined theoretically from known nuclear data. Such computations are based on the inventory of nuclei created during the fission process and after reactor shutdown and their radioactive decay characteristics:where fðtÞ is the power function, E i is the mean decay energy of the ith nuclide ( , , and components), i is the decay constant of the ith nuclide, and N i ðtÞ is the number of nuclide i at cooling time t. These calculations require extensive libraries of cross sections, fission yields, and decay data. Obviously, an accurate assessment of the decay heat is highly relevant...
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Two complementary experimental techniques have been used to extract precise branching ratios to unbound states in 12 C from 12 N and 12 B β-decays. In the first the three α-particles emitted after βdecay are measured in coincidence in separate detectors, while in the second method 12 N and 12 B are implanted in a detector and the summed energy of the three α-particles is measured directly. For the narrow states at 7.654 MeV (0 +) and 12.71 MeV (1 +) the resulting branching ratios are both smaller than previous measurements by a factor of 2. The experimental results are compared to no-core shell model calculations with realistic interactions from chiral perturbation theory, and inclusion of three-nucleon forces is found to give improved agreement.
The β decays of 12 N and 12 B have been studied at KVI and JYFL to resolve the composition of the broad and interfering 0 + and 2 + strengths in the triple-α continuum. For the first time a complete treatment of 3α decay is presented including all major breakup channels. A multilevel, many-channel R-matrix formalism has been developed for the complete description of the breakup in combination with the recently published separate analysis of angular correlations. We find that, in addition to the Hoyle state at 7.65 MeV, more than one 0 + and 2 + state is needed to reproduce the spectra. Broad 0 + 3 and 2 + 2 states are found between 10.5 and 12 MeV in this work. The presence of β strength up to the 12 N Q-value window suggests the presence of additional 0 + and 2 + components in the 12 C structure at energies above 12.7 MeV.
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