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We report the first measurement of the neutron cross section on argon in the energy range of 100-800 MeV. The measurement was obtained with a 4.3-hour exposure of the Mini-CAPTAIN detector to the WNR/LANSCE beam at LANL. The total cross section is measured from the attenuation coefficient of the neutron flux as it traverses the liquid argon volume. A set of 2,631 candidate interactions is divided in bins of the neutron kinetic energy calculated from time-offlight measurements. These interactions are reconstructed with custom-made algorithms specifically designed for the data in a time projection chamber the size of the Mini-CAPTAIN detector. The energy averaged cross section is 0.91 ± 0.10 (stat.) ± 0.09 (sys.) barns. A comparison of the measured cross section is made to the GEANT4 and FLUKA event generator packages, where the energy averaged cross sections in this range are 0.60 and 0.68 barns respectively.

Airborne gamma-ray surveys are useful for many applications, ranging from geology and mining to public health and nuclear security. In all these contexts, the ability to decompose a measured spectrum into a linear combination of background source terms can provide useful insights into the data and lead to improvements over techniques that use spectral energy windows. Multiple methods for the linear decomposition of spectra exist but are subject to various drawbacks, such as allowing negative photon fluxes or requiring detailed Monte Carlo modeling. We propose using Non-negative Matrix Factorization (NMF) as a data-driven approach to spectral decomposition. Using aerial surveys that include flights over water, we demonstrate that the mathematical approach of NMF finds physically relevant structure in aerial gamma-ray background, namely that measured spectra can be expressed as the sum of nearby terrestrial emission, distant terrestrial emission, and radon and cosmic emission. These NMF background components are compared to the background components obtained using Noise-Adjusted Singular Value Decomposition (NASVD), which contain negative photon fluxes and thus do not represent emission spectra in as straightforward a way. Finally, we comment on potential areas of research that are enabled by NMF decompositions, such as new approaches to spectral anomaly detection and data fusion.

Networked detector systems can be deployed in urban environments to aid in the detection and localization of radiological and/or nuclear material. However, effectively responding to and interpreting a radiological alarm using spectroscopic data alone may be hampered by a lack of situational awareness, particularly in complex environments. This study investigates the use of LiDAR and streaming video to enable real-time object detection and tracking, and the fusion of this tracking information with radiological data for the purposes of enhanced situational awareness and increased detection sensitivity. This work presents a novel object detection, tracking, and source-object attribution analysis that is capable of operating in real-time. By implementing this analysis pipeline on a custom developed system that comprises a static 2 × 4 × 16 inch NaI(Tl) detector co-located with a 64-beam LiDAR and 4 monocular cameras, we demonstrate the ability to accurately correlate trajectories from tracked objects to spectroscopic gamma-ray data in real time, and use physics-based models to reliably discriminate between source-carrying and non-source-carrying objects. In this work, we describe our approach in detail and present a quantitative performance assessment that characterizes the source-object attribution capabilities of both video and Li-DAR. Additionally, we demonstrate the ability to simultaneously track pedestrians and vehicles in a mock urban environment, and use this tracking information to improve both detection sensitivity and situational awareness using our contextual-radiological data fusion methodology.

Artificial neural networks (ANNs) for performing spectroscopic gamma-ray source identification have been previously introduced, primarily for applications in controlled laboratory settings. To understand the utility of these methods in scenarios and environments more relevant to nuclear safety and security, this work examines the use of ANNs for mobile detection, which involves highly variable gamma-ray background, low signal-to-noise ratio measurements, and low false alarm rates. Simulated data from a 2” × 4” × 16” NaI(Tl) detector are used in this work for demonstrating these concepts, and the minimum detectable activity (MDA) is used as a performance metric in assessing model performance.In addition to examining simultaneous detection and identification, binary spectral anomaly detection using autoencoders is introduced in this work, and benchmarked using detection methods based on Non-negative Matrix Factorization (NMF) and Principal Component Analysis (PCA). On average, the autoencoder provides a 12% and 23% improvement over NMF- and PCA-based detection methods, respectively. Additionally, source identification using ANNs is extended to leverage temporal dynamics by means of recurrent neural networks, and these time-dependent models outperform their time-independent counterparts by 17% for the analysis examined here. The paper concludes with a discussion on tradeoffs between the ANN-based approaches and the benchmark methods examined here.

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