Abstract. The intensification of thaw-driven mass wasting is transforming glacially conditioned permafrost terrain, coupling slopes with aquatic systems, and triggering a cascade of downstream effects. Within the context of recent, rapidly evolving climate controls on the geomorphology of permafrost terrain, we (A) quantify three-dimensional retrogressive thaw slump enlargement and describe the processes and thresholds coupling slopes to downstream systems, (B) investigate catchment-scale patterns of slope thermokarst impacts and the geomorphic implications, and (C) map the propagation of effects through hydrological networks draining permafrost terrain of northwestern Canada. Power-law relationships between retrogressive thaw slump area and volume (R2=0.90), as well as the thickness of permafrost thawed (R2=0.63), combined with the multi-decadal (1986–2018) increase in the areal extent of thaw slump disturbance, show a 2 order of magnitude increase in catchment-scale geomorphic activity and the coupling of slope and hydrological systems. Predominant effects are to first- and second-order streams where sediment delivery, often indicated by formation of recent debris tongue deposits, commonly exceeds the transport capacity of headwater streams by orders of magnitude, signaling centennial- to millennial-scale perturbation of downstream systems. Assessment of hydrological networks indicates that thaw-driven mass wasting directly affects over 5538 km of stream segments, 889 km of coastline, and 1379 lakes in the 994 860 km2 study area. Downstream propagation of slope thermokarst indicates a potential increase in the number of affected lakes by at least a factor of 4 (n>5692) and impacted stream length by a factor of 8 (>44 343 km), and it defines several major impact zones on lakes, deltas, and coastal areas. Prince of Wales Strait is the receiving marine environment for greatly increased sediment and geochemical fluxes from numerous slump-impacted hydrological networks draining Banks Island and Victoria Island. The Peel and Mackenzie rivers are globally significant conveyors of the slope thermokarst cascade, delivering effects to North America's largest Arctic delta and the Beaufort Sea. Climate-driven erosion of ice-rich slopes in permafrost-preserved glaciated terrain has triggered a time-transient cascade of downstream effects that signal the rejuvenation of post-glacial landscape evolution. Glacial legacy, ground-ice conditions, and continental drainage patterns dictate that terrestrial, freshwater, coastal, and marine environments of western Arctic Canada will be an interconnected hotspot of thaw-driven change through the coming millennia.

Abstract. The intensification of thaw-driven mass wasting is transforming glacially-conditioned permafrost terrain, coupling slopes with aquatic systems, and triggering a cascade of downstream effects. Within the context of recent, rapidly evolving climate controls on the geomorphology of permafrost terrain we: A) quantify three-dimensional slump enlargement and described the processes and thresholds coupling slopes to downstream systems; B) investigate catchment-scale patterns of slope thermokarst (thaw slumps and slides) impacts and the geomorphic implications; and C) project the propagation of effects through hydrological networks draining continuous permafrost of northwestern Canada. Power-law relationships between thaw-slump area and volume (R2 = 0.90), and thickness of permafrost thawed (R2 = 0.63), combined with the multi-decadal (1985–2018) increase in areal extent of thaw-slump disturbance show a two-order of magnitude increase in catchment-scale geomorphic activity and the coupling of slope and hydrological systems. Predominant catchment effects are to first- and second-order streams where sediment delivery commonly exceeds stream transport capacity by orders of magnitude indicating millennial-scale perturbation of downstream systems. Assessment of hydrological networks indicates thaw-driven mass wasting directly affects over 6,760 km of stream segments, 890 km of coastline, and 1,370 lakes in the 994,860 km2 study area. Downstream propagation of slope thermokarst indicates a potential increase in the number of affected lakes by at least a factor of 4 (n > 5,600), impacted stream length by a factor of 7 (> 48,000 km) and defines several major impact zones to lakes, deltas, and coastal areas. Prince of Wales Strait is the receiving marine environment for greatly increased sediment and geochemical fluxes from numerous slump impacted hydrological networks draining the landmasses of Banks and Victoria Islands. Peel and Mackenzie Rivers are globally significant conveyors of the slope thermokarst cascade delivering effects to North America’s largest Delta and the Beaufort Sea. Climate-driven erosion of ice-rich slopes in permafrost preserved glaciated terrain has triggered a time-transient cascade of downstream effects that signal the renewal of post-glacial landscape evolution. Glacial legacy and the patterns of continental drainage dictate that terrestrial, freshwater and marine environments of western Arctic Canada will be an interconnected hotspot of thaw-driven change through the coming millennia.

Abstract. As climate warming and precipitation increase at high latitudes, permafrost terrains across the circumpolar north are poised for intensified geomorphic activity and sediment mobilization that are expected to persist for millennia. In previously glaciated permafrost terrain, ice-rich deposits are associated with large stores of reactive mineral substrate. Over geological timescales, chemical weathering moderates atmospheric CO2 levels, raising the prospect that mass wasting driven by terrain consolidation following thaw (thermokarst) may enhance weathering of permafrost sediments and thus climate feedbacks. The nature of these feedbacks depends upon the mineral composition of sediments (weathering sources) and the balance between atmospheric exchange of CO2 vs. fluvial export of carbonate alkalinity (Σ[HCO3-, CO32-]). Working in the fluvially incised, ice-rich glacial deposits of the Peel Plateau in northwestern Canada, we determine the effects of slope thermokarst in the form of retrogressive thaw slump (RTS) activity on mineral weathering sources, CO2 dynamics, and carbonate alkalinity export and how these effects integrate across watershed scales (∼ 2 to 1000 km2). We worked along three transects in nested watersheds with varying connectivity to RTS activity: a 550 m transect along a first-order thaw stream within a large RTS, a 14 km transect along a stream which directly received inputs from several RTSs, and a 70 km transect along a larger stream with headwaters that lay outside of RTS influence. In undisturbed headwaters, stream chemistry reflected CO2 from soil respiration processes and atmospheric exchange. Within the RTS, rapid sulfuric acid carbonate weathering, prompted by the exposure of sulfide- and carbonate-bearing tills, appeared to increase fluvial CO2 efflux to the atmosphere and propagate carbonate alkalinity across watershed scales. Despite covering less than 1 % of the landscape, RTS activity drove carbonate alkalinity to increase by 2 orders of magnitude along the largest transect. Amplified export of carbonate alkalinity together with isotopic signals of shifting DIC and CO2 sources along the downstream transects highlights the dynamic nature of carbon cycling that may typify glaciated permafrost watersheds subject to intensification of hillslope thermokarst. The balance between CO2 drawdown in regions where carbonic acid weathering predominates and CO2 release in regions where sulfides are more prevalent will determine the biogeochemical legacy of thermokarst and enhanced weathering in northern permafrost terrains. Effects of RTSs on carbon cycling can be expected to persist for millennia, indicating a need for their integration into predictions of weathering–carbon–climate feedbacks among thermokarst terrains.

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<p>Recent intensification of slope thermokarst is transforming permafrost preserved glaciated landscapes and causing significant downstream effects. In this paper we: A) Describe the thaw-related mechanisms driving the evolution of slope to stream connectivity; B) define the watershed patterns of thermokarst intensification; and C) project the cascade of effects through the Arctic drainage networks of northwestern Canada. The power-law relationships between disturbance area and volume, and thickness of permafrost thawed, in conjunction with a time-series of disturbance mapping show that the non-linear intensification of slope thermokarst is mobilizing vast stores of previously frozen glacial sediments linking slopes to downstream systems. Mapping across a range of catchment scales indicates that slope thermokarst predominantly affects first and second order streams. Slope sediment delivery now frequently exceeds fluvial transport capacity of these streams by several orders of magnitude indicating long-term perturbation. Mapping shows slope thermokarst is directly affecting over 6760 km of stream segments, over 890 km of coastline and over 1370 lakes across the 1,000,000 km<sup>2</sup> Arctic drainage basin from continuous permafrost of northwestern Canada. The downstream projection of thermokarst disturbance increases affected lakes by a factor of 4 and stream length by a factor of 7, and suggests that fluvial transfer has the potential to yield numerous thermokarst impact zones across coastal areas of western Arctic Canada. The Prince of Wales Strait between Banks and Victoria Islands is identified as a hotspot of downstream thermokarst effects, and the Peel and Mackenzie rivers stand out as principle conveyors of slope thermokarst effects to North America’s largest Delta and to the Beaufort Sea.<strong> </strong>The distribution of slope thermokarst and the fluvial pattern of sediment mobilization signal the climate-driven rejuvenation of post-glacial landscape change and the triggering of a time-transient cascade of downstream effects. Geological legacy and the patterns of continental drainage dictate that terrestrial, freshwater and marine environments of western Arctic Canada will be a hotspot of climate-driven change through the coming centuries. </p>

Abstract. The chemical weathering of minerals is a primary control on atmospheric CO2 levels and Earth's climate over geological timescales. As climate warming and precipitation intensify at high latitudes, glaciated terrains across the circumpolar north are poised for rapid geomorphic change and associated changes in mineral weathering dynamics. Here, we determine how the effects of permafrost thaw on mineral weathering sources and inorganic carbon cycling and export integrate across watershed scales (from ~ 2 to 1000 km2) in a permafrost terrain within a former glacial margin and dominated by relatively inorganic sediments (Peel Plateau, Canada). Our work was conducted along three nested transects with varying intensities of retrogressive thaw slump (RTS) thermokarst activity: a 550 m transect along a first-order thaw stream within a RTS; a 14 km transect along a stream which directly received RTS inputs; and a 70 km transect along a larger stream which received inputs from RTS-affected tributaries. In the thaw stream, rapid sulfuric acid weathering of carbonate tills appeared to amplify CO2 efflux to the atmosphere and HCO3− export downstream, where DIC and CO2 stable isotopes revealed a shift to an abiotic-inorganic driven aquatic carbon cycle. Along the intermediate transect, DIC concentrations were ten times higher in the RTS-affected reach than in the undisturbed headwaters, and decreased downstream with decreasing RTS area. Along the largest transect, HCO3− concentrations increased by two orders of magnitude in association with RTS activity, despite RTSs covering only ~ 0.5 % of the landscape. Statistical modeling of hydrochemical measurements and geospatial landscape data showed that RTSs were a primary landscape driver of HCO3− export across watershed scales. Constraining sources and rates of mineral weathering across diverse permafrost terrains will help to understand future changes in Arctic aquatic carbon cycling, as our results suggest that abiotic-inorganic processes may become prevalent.

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