Hybrid supercapacitors have been regarded as next-generation energy storage devices due to their outstanding performances. However, hybrid supercapacitors remain a great challenge to enhance the energy density of hybrid supercapacitors. Herein, a novel approach for high-energy density hybrid supercapacitors based on a laser scribed graphene cathode and AlPO4-carbon hybrid coated H2Ti12O25 (LSG/H-HTO) was designed. Benefiting from high-energy laser scribed graphene and high-power H-HTO, it was demonstrated that LSG/H-HTO delivers superior energy and power densities with excellent cyclability. Compared to previous reports on other hybrid supercapacitors, LSG/H-HTO electrode composition shows extraordinary energy densities of ~70.8 Wh/kg and power densities of ~5191.9 W/kg. Therefore, LSG/H-HTO can be regarded as a promising milestone in hybrid supercapacitors.

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The emergence of organic electrochemical transistors (OECTs) has opened a new era of printable electronics and bioelectronics, due to their unique advantages including innately superior transconductance and biocompatibility. Despite the foreseeable advancements available from their further implementations in fundamental logic circuitry, however, insufficient operation speeds and short compatibilities to scaling‐down have so far hindered advanced integrations other than biosensing and biosignal amplifications. Here, a 3D‐construction‐dependent operational analysis of OECTs is reported, with which an all‐vertical architectural design enabled unprecedentedly high operating speed and a facile expansion to large‐area and high‐density 3D crossbar arrays. A simple vertical channel architecture completed with solid‐state Ag/AgCl top‐gate electrodes enables an ultrafast redistribution of ions within channels, yielding a state‐of‐the‐art operation frequency reaching 12 MHz V−1. Various printed logic circuit arrays, including NOT, NAND, and NOR gates, with high stability and reproducibility.