[1] Time series measurements of the nuclear fuel reprocessing tracers, 129 I and 137 Cs, and ventilation tracer, CFC-11, were used to determine circulation time scales for Atlantic Water (AW) in the Arctic Ocean. Measurements in surface water are consistent with an advection model and transit times from the North Sea of 1-4 years to the Barents Sea, 3-6 years to the Kara Sea, and 9-12 years to the North Pole.
Anthropogenic radionuclides released into European coastal waters from nuclear fuel reprocessing plants at Sellafield (UK) and La Hague (France) flow northward through the Nordic Seas and label Atlantic Water (AW) entering the Arctic Ocean. Transport of the soluble radionuclide 129I through the Arctic Ocean has been simulated using a numerical model for the period from 1970 to 2010. The simulated tracer distributions closely conform to 129I measurements made across the Arctic Ocean during the mid‐1990s and 2000s and clearly illustrate the dramatic changes in oceanic circulation which occurred during this time. The largest changes in surface circulation were associated with the transition from a negative to a positive phase of the Arctic Oscillation in the early 1990s and the subsequent return to a weak positive phase in the late 1990s and early 2000s. Model and experimental results indicate that a new circulation regime evolved after 2004 when a period of intense, anti‐cyclonic surface stress led to a strengthening of the Beaufort Gyre. We submit that this resulted in a suppression of the cyclonic boundary current of mid‐depth Atlantic Water (AW) below the Beaufort Gyre, with upper AW in the Canada Basin showing signs of a reversal from cyclonic to anti‐cyclonic flow. These results are consistent with the development of a new AW circulation scheme involving a separation between flow at intermediate depths in the Eurasian and Canada Basins which could eventually result in modification of the Arctic intermediate water which feeds the overflows.
The events that followed the Tohoku earthquake and tsunami on March 11, 2011, included the loss of power and overheating at the Fukushima Daiichi nuclear power plants, which led to extensive releases of radioactive gases, volatiles, and liquids, particularly to the coastal ocean. The fate of these radionuclides depends in large part on their oceanic geochemistry, physical processes, and biological uptake. Whereas radioactivity on land can be resampled and its distribution mapped, releases to the marine environment are harder to characterize owing to variability in ocean currents and the general challenges of sampling at sea. Five years later, it is appropriate to review what happened in terms of the sources, transport, and fate of these radionuclides in the ocean. In addition to the oceanic behavior of these contaminants, this review considers the potential health effects and societal impacts.
The magnitude of the flux of biogenic particulate organic carbon (POC) exported from the surface waters of the world ocean and remineralized at depth is critical to constraining models of the global carbon cycle, yet remains controversial. The use of upper ocean sediment traps is still one of the primary tools for determining this export flux, although trap fluxes have been shown to vary significantly because of hydrodynamic and sample collection biases. Over the past decade, 234 Th increasingly has been used as a tracer to estimate POC export from the euphotic zone by multiplying the depth-integrated 234 Th flux by the POC/ 234 Th ratio of sinking particles. The accuracy of this technique is highly dependent on the natural variability in the POC/ 234 Th ratio and 234 Th flux, yet the significance of this variability to estimates of POC export remains uncertain. Based on an analysis of new 234 Th and POC data from the Labrador Sea and a review of 25 previous independent field studies, we report that POC export fluxes can vary 2-10 times or more solely because of variability in the POC/ 234 Th ratio and procedures used to estimate the 234 Th flux. Recommended improvements include studies of the biological, chemical, and physical mechanisms controlling 234 Th-organic matter interactions in seawater; detailed comparisons of POC/ 234 Th ratios in size-fractionated and sediment trap material; increased spatial and temporal sampling density of 234 Th; and more standardized procedures to calculate the 234 Th export flux.
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